Identification and Screening of Trace and Multityped Solvents Using Transpiration-Driven Electrokinetic Generation Principle
2025
发表期刊NANO LETTERS (IF:9.6[JCR-2023],10.1[5-Year])
ISSN1530-6984
EISSN1530-6992
卷号25期号:6页码:2396-2403
发表状态已发表
DOI10.1021/acs.nanolett.4c05840
摘要

Transpiration-driven electrokinetic power generators (TEPGs) hold promising potential for intelligent chemical sensing applications, enabling the efficient identification and screening of organic solvents. Here, we report a novel TEPG-based chemical sensor using MoS2-doped cellulose filter paper for efficient detection of poplar solvents like water, alcohols, and methanol. TEPGs operate by leveraging capillary-driven transpiration to induce solvent flow through porous materials, leading to ion migration and the formation of electrical double layers (EDLs) at the solid-liquid interfaces. This process generates a potential difference, enabling the conversion of the mechanical transpiration energy into electrical signals. Integrated with machine learning algorithms and IoT technologies, the sensor achieves real-time classification of the solvents. This TEPG-CS system offers enhanced sensitivity, reliability, and operational adaptability, overcoming the limitations of the traditional detection methods. This work has broad potential for environmental monitoring, industrial applications, and biomedical fields, offering another pathway for advanced solvent detection and classification systems.

关键词transpiration-driven electrokinetic power generators polar solvents detection machine learning MoS2-doped cellulose solvent recognition sensors
URL查看原文
收录类别SCI ; EI
语种英语
资助项目National Natural Science Foundation of China[
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS类目Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS记录号WOS:001413011500001
出版者AMER CHEMICAL SOC
EI入藏号20250617804618
EI主题词Electrogasdynamic power generation
EI分类号101.8 Biosensing Technology ; 301.1.2 Gas Dynamics ; 301.2.2 Electrohydrodynamics ; 802 Chemical Apparatus and Plants ; Unit Operations ; Unit Processes ; 802.2 Chemical Reactions ; 802.3 Chemical Operations ; 803 Chemical Agents and Basic Industrial Chemicals ; 804 Chemical Products
原始文献类型Journal article (JA)
文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/487130
专题物质科学与技术学院
物质科学与技术学院_PI研究组_凌盛杰组
物质科学与技术学院_硕士生
物质科学与技术学院_博士生
物质科学与技术学院_PI研究组_刘一凡组
通讯作者Ren, Jing; Ling, Shengjie
作者单位
1.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
2.Fudan Univ, Dept Macromol Sci, Shanghai 200433, Peoples R China
3.Fudan Univ, State Key Lab Mol Engn Polymers, Dept Macromol Sci, Shanghai 200433, Peoples R China
4.Fudan Univ, Res Ctr AI Polymer Sci, Dept Macromol Sci, Shanghai 200433, Peoples R China
5.ShanghaiTech Univ, State Key Lab Adv Med Mat & Devices, Shanghai 201210, Peoples R China
6.Shanghai Clin Res & Trial Ctr, Shanghai 201210, Peoples R China
第一作者单位物质科学与技术学院
通讯作者单位物质科学与技术学院;  上海科技大学
第一作者的第一单位物质科学与技术学院
推荐引用方式
GB/T 7714
Gao, Wenli,Yu, Mengfei,Cao, Leitao,et al. Identification and Screening of Trace and Multityped Solvents Using Transpiration-Driven Electrokinetic Generation Principle[J]. NANO LETTERS,2025,25(6):2396-2403.
APA Gao, Wenli.,Yu, Mengfei.,Cao, Leitao.,Wen, Piao.,Sun, Yi.,...&Ling, Shengjie.(2025).Identification and Screening of Trace and Multityped Solvents Using Transpiration-Driven Electrokinetic Generation Principle.NANO LETTERS,25(6),2396-2403.
MLA Gao, Wenli,et al."Identification and Screening of Trace and Multityped Solvents Using Transpiration-Driven Electrokinetic Generation Principle".NANO LETTERS 25.6(2025):2396-2403.
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