Ferrimagnetic Kitaev spin liquids in mixed spin 1/2 spin 3/2 honeycomb magnets
2024-12-12
状态已发表
摘要We explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr0.5Ru0.5Cl3, where spin-1/2 and spin-3/2 ions occupy distinct sublattices of a honeycomb lattice. By developing a superexchange theory specifically for this mixed-spin system, we identify the conditions under which dominant Kitaev-like interactions emerge. Focusing on the limiting case of pure Kitaev coupling with single-ion anisotropy, we employ a combination of superexchange theory, par ton mean-field theory, and density matrix renormalization group (DMRG) simulations. We establish a comprehensive ground-state phase diagram identifying four distinct quantum spin liquid phases. Our findings highlight the importance of spin-orbital couplings and quadrupolar order parameters in stabilizing exotic phases, providing a foundation for exploring mixed-spin Kitaev magnets.
语种英语
DOIarXiv:2412.09310
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出处Arxiv
收录类别PPRN.PPRN
WOS记录号PPRN:119900102
WOS类目Physics, Condensed Matter
资助项目US Department of Energy Basic Energy Sciences[DE-SC0020330] ; Deutsche Forschungsgemeinschaft (DFG, German Research Foundation)["EXC–2111–390814868","KN1254/1-2","KN1254/2-1","TRR 360-492547816"] ; National Science Foundation["DMR-1929311","PHY-2210452"]
文献类型预印本
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/483973
专题物质科学与技术学院
物质科学与技术学院_PI研究组_金汇可组
通讯作者Natori, Willian
作者单位
1.Univ Campinas, Gleb Wataghin Inst Phys, BR-13083950 Campinas, SP, Brazil
2.Inst Laue Langevin, BP 156,41 Ave Martyrs, F-38042 Grenoble, France
3.Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455, USA
4.Univ Virginia, Dept Phys, Charlottesville, VA 22904, USA
5.Tech Univ Munich, TUM Sch Nat Sci, Phys Dept, D-85748 Garching, Germany
6.Munich Ctr Quantum Sci & Technol MCQST, Schellingstr 4, D-80799 Munich, Germany
7.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
8.Imperial Coll London, Blackett Lab, London SW7 2AZ, England
推荐引用方式
GB/T 7714
Natori, Willian,Yang, Yang,Jin, Hui-Ke,et al. Ferrimagnetic Kitaev spin liquids in mixed spin 1/2 spin 3/2 honeycomb magnets. 2024.
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