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Design, Preparation, and Solvent Identification Application of Antheraea pernyi Silk Paper-based Electrochemical Sensor | |
其他题名 | Design,Preparation,and Solvent Identification Application of Antheraea pernyi Silk Paper-based Electrochemical Sensor |
2024-08 | |
发表期刊 | ACTA POLYMERICA SINICA (IF:1.7[JCR-2023],1.3[5-Year]) |
ISSN | 1000-3304 |
EISSN | 1000-3304 |
卷号 | 55期号:8页码:954-965 |
发表状态 | 已发表 |
DOI | 10.11777/j.issn1000-3304.2024.24050 |
摘要 | This study focuses on the development of a sustainable and highly sensitive Antheraea pernyi (A. pernyi) silk paper-based electrochemical sensor, utilizing the excellent solvent resistance of silk paper as the substrate and incorporating molybdenum disulfide (MoS2) functional units. The electrochemical sensing principle of this sensor is based on a transpiration-driven electricity generation mechanism. Different solvents interact distinctly with the sensor, resulting in transpiration-driven electrical signals with varying characteristics. Although these electrical signals display complex band-shaped patterns lacking sharp peaks or specific mutation points, they exhibit highly reproducible trends for specific solvent systems. Consequently, this study further employs a feedforward neural network to construct a solvent identification model based on the oak silk fibroin ultrafine paper electrochemical sensor. This model processes and analyzes these complex yet highly repetitive electrical signals. The AI-driven A. pernyi silk paper-based electrochemical sensor not only accurately identifies solvents with highly similar chemical structures and properties, such as methanol, ethanol, isopropanol, and deionized water, but also recognizes chemically similar mixed solvent systems, like varying proportions of ethanol-water mixtures. In 100 identification tests, the accuracy was 100%. The development of this AI-driven A. pernyi silk paper-based electrochemical sensor offers a convenient, cost-effective method for rapid and accurate solvent detection, holding significant implications in fields such as alcohol testing, environmental monitoring, and chemical analysis. |
关键词 | Silk paper Eutectic solvent Depolymerization Electrochemical sensor Deep learning |
URL | 查看原文 |
收录类别 | SCI ; 中国科技核心期刊 ; 北大核心 ; SCIE ; CSCD |
语种 | 中文 |
WOS研究方向 | Polymer Science |
WOS类目 | Polymer Science |
WOS记录号 | WOS:001315124600003 |
出版者 | SCIENCE PRESS |
原始文献类型 | Periodical |
来源库 | WanFang |
文献类型 | 期刊论文 |
条目标识符 | https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/427460 |
专题 | 物质科学与技术学院 物质科学与技术学院_PI研究组_凌盛杰组 物质科学与技术学院_硕士生 物质科学与技术学院_博士生 物质科学与技术学院_PI研究组_刘一凡组 |
通讯作者 | Zheng, Ke; Gao, Wen-li; Ling, Sheng-jie |
作者单位 | 1.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China 2.Anhui Agr Univ, Sch Mat Sci & Chem, Hefei 230023, Peoples R China 3.ShanghaiTech Univ, State Key Lab Adv Med Mat & Devices, Shanghai, Peoples R China 4.Shanghai Clin Res & Trial Ctr, Shanghai 201210, Peoples R China |
第一作者单位 | 物质科学与技术学院 |
通讯作者单位 | 物质科学与技术学院; 上海科技大学 |
第一作者的第一单位 | 物质科学与技术学院 |
推荐引用方式 GB/T 7714 | Sun, Yi,Wu, Wei,Wen, Piao,et al. Design, Preparation, and Solvent Identification Application of Antheraea pernyi Silk Paper-based Electrochemical Sensor[J]. ACTA POLYMERICA SINICA,2024,55(8):954-965. |
APA | Sun, Yi.,Wu, Wei.,Wen, Piao.,Ren, Jing.,Zheng, Ke.,...&Ling, Sheng-jie.(2024).Design, Preparation, and Solvent Identification Application of Antheraea pernyi Silk Paper-based Electrochemical Sensor.ACTA POLYMERICA SINICA,55(8),954-965. |
MLA | Sun, Yi,et al."Design, Preparation, and Solvent Identification Application of Antheraea pernyi Silk Paper-based Electrochemical Sensor".ACTA POLYMERICA SINICA 55.8(2024):954-965. |
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