上海科技大学知识管理系统

Blackbody-sensitive uncooled infrared photodetectors with ultra-broadband and ultrafast photoresponse have a profound impact on many areas of modern science and technology. However, it is a big challenge for both traditional photodetectors and emerging low-dimensional ones to simultaneously have all the above characteristics. Here, this challenge is addressed by establishing a Te/WTe2 heterostructure photodetector. The built-in field of the heterostructure and the crossing conduction and valence bands of WTe2 jointly result in a high responsivity and a visible-to-long-wavelength-infrared photoresponse range. The peak responsivity (at the 3.3 µm wavelength) reaches 914 mA W−1 at zero bias and 8.51 A W−1 at 2 V bias. Further, the joint action coupled with the high mobility of Te and WTe2 promotes the 3-dB bandwidth to 153 kHz. The self-powered blackbody responsivity and specific detectivity reach 235.7 mA W−1 and 1.1 × 108 cm Hz1/2 W−1, respectively. The former increases to 5.82 A W−1 at 1 V bias. Moreover, this device is polarization-sensitive with a contrast ratio of 2. This work reveals the potential of the Te/WTe2 heterostructure for high-performance room-temperature infrared photodetectors. © 2024 Wiley-VCH GmbH.