Disorder-induced broadening of the spin waves in a triangular-lattice quantum-spin-liquid candidate YbZnGaO4
2022-02-11
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摘要

Disorder is important in the study of quantum spin liquids, but its role on the spin dynamics remains elusive. Here, we explore the disorder effect by investigating the magnetic-field dependence of the low-energy magnetic excitations in a triangular-lattice frustrated magnet YbZnGaO4 with inelastic neutron scattering. With an intermediate field of 2.5 T applied along the c-axis, the broad continuum at zero field becomes more smeared both in energy and momentum. With a field up to 10 T, which fully polarizes the magnetic moments, we observe clear spin-wave excitations with a gap of ∼1.4 meV comparable to the bandwidth. However, the spectra are significantly broadened. The excitation spectra both at zero and high fields can be reproduced by performing classical Monte Carlo simulations which take into account the disorder effect arising from the random site mixing of nonmagnetic Zn2+ and Ga3+ ions. These results elucidate the critical role of disorder in broadening the magnetic excitation spectra and mimicking the spin-liquid features in frustrated quantum magnets.

DOIarXiv:2202.05462
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出处Arxiv
WOS记录号PPRN:12066737
WOS类目Physics, Condensed Matter
资助项目National Key Projects for Research and Development of China[
文献类型预印本
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/348539
专题物质科学与技术学院
生命科学与技术学院_硕士生
物质科学与技术学院_公共科研平台_拓扑物理实验室
免疫化学研究所_公共科研平台_生物医学大数据平台
物质科学与技术学院_PI研究组_张石磊组
作者单位
1.Hubei Normal Univ, Inst Adv Mat, Huangshi 435002, Peoples R China
2.Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Peoples R China
3.Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Peoples R China
4.Nanjing Univ, Dept Phys, Nanjing 210093, Peoples R China
5.Nanjing Univ Sci & Technol, Dept Appl Phys, Nanjing 210094, Peoples R China
6.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 200031, Peoples R China
7.ShanghaiTech Univ, ShanghaiTech Lab Topol Phys, Shanghai 200031, Peoples R China
8.Nanjing Univ Posts & Telecommun, Sch Sci, Nanjing 210023, Peoples R China
9.Inst Laue Langevin, 71 Ave Martyrs, F-38042 Grenoble, France
10.Forschungszent Julich, Julich Ctr Neutron Sci JCNS, Heinz Maier Leibnitz Zent MLZ, Lichtenbergstr 1, D-85747 Garching, Germany
推荐引用方式
GB/T 7714
Ma, Zhen,Dong, Zhao-Yang,Wang, Jinghui,et al. Disorder-induced broadening of the spin waves in a triangular-lattice quantum-spin-liquid candidate YbZnGaO4. 2022.
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