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Molten-Salt Synthesis of Triazine-Based Carbon Nitride and Its Photocatalytic Degradation Mechanism Investigation by In Situ NMR
2023-05-01
发表期刊JOURNAL OF PHYSICAL CHEMISTRY C (IF:3.3[JCR-2023],3.5[5-Year])
ISSN1932-7447
EISSN1932-7455
卷号127期号:18页码:8687-8694
发表状态已发表
DOI10.1021/acs.jpcc.3c01631
摘要Carbon nitride-based catalysts are nonmetallic materi-als with efficient photocatalysis for water splitting, degradation of organic dyes, and CO2 reduction. In this paper, a one-step molten salt method was employed for the synthesis of ionic doped carbon nitride materials named CNs (carbon nitride catalysts), which exhibited excellent adsorption performance and photocatalytic activity. The adulteration of Zn2+ ions created a unique nanosheet stack morphology, leading to more effective active sites and better electron transfer efficiency. Additionally, the degradation mechanism was investigated by the quasi-in situ NMR method. The reaction products and photocatalytic process were fully discussed, providing a new degradative pathway of methylene blue (MB) by such CN-based
关键词Carbon nitride Catalysts Degradation Fused salts Molten materials Nuclear magnetic resonance spectroscopy Photocatalytic activity Adsorption performance Adsorption-photocatalytic CO 2 reduction Degradation of organic dyes Mechanism investigation Molten salts synthesis Molten-salts method Photocatalytic degradation mechanism Water splitting ]+ catalyst
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收录类别SCI ; EI
语种英语
资助项目National Natural Science Foundation of China["22103094","21904088"]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science
WOS类目Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号WOS:000984342200001
出版者AMER CHEMICAL SOC
EI入藏号20232114116466
EI主题词Aromatic compounds
EI分类号801.4 Physical Chemistry ; 802.2 Chemical Reactions ; 803 Chemical Agents and Basic Industrial Chemicals ; 804 Chemical Products Generally ; 804.1 Organic Compounds ; 804.2 Inorganic Compounds
原始文献类型Journal article (JA)
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文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/305006
专题iHuman研究所
iHuman研究所_公共科研平台_生命科学NMR平台
通讯作者Fu, Xiaobin; Liu, Hongtao
作者单位
1.Chinese Acad Sci, Shanghai Inst Appl Phys, Key Lab Interfacial Phys & Technol, Shanghai 201800, Peoples R China
2.ShanghaiTech Univ, iHuman Inst, Shanghai 201210, Peoples R China
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GB/T 7714
Yingsu, Junheng,Liu, Yiyang,Huang, Hailong,et al. Molten-Salt Synthesis of Triazine-Based Carbon Nitride and Its Photocatalytic Degradation Mechanism Investigation by In Situ NMR[J]. JOURNAL OF PHYSICAL CHEMISTRY C,2023,127(18):8687-8694.
APA Yingsu, Junheng.,Liu, Yiyang.,Huang, Hailong.,Yang, Lingyun.,Qian, Yuan.,...&Liu, Hongtao.(2023).Molten-Salt Synthesis of Triazine-Based Carbon Nitride and Its Photocatalytic Degradation Mechanism Investigation by In Situ NMR.JOURNAL OF PHYSICAL CHEMISTRY C,127(18),8687-8694.
MLA Yingsu, Junheng,et al."Molten-Salt Synthesis of Triazine-Based Carbon Nitride and Its Photocatalytic Degradation Mechanism Investigation by In Situ NMR".JOURNAL OF PHYSICAL CHEMISTRY C 127.18(2023):8687-8694.
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