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| Facile Solvent-free Synthesis of Hollow Fiber Catalyst Assembled by c-axis Oriented ZSM-5 Crystals | |
| 2018-12-21 | |
| 发表期刊 | CHEMCATCHEM (IF:3.8[JCR-2023],4.6[5-Year]) |
| ISSN | 1867-3880 |
| 卷号 | 10期号:24页码:5619-5626 |
| 发表状态 | 已发表 |
| DOI | 10.1002/cctc.201801517 |
| 摘要 | Well crystallized hollow fibers assembled by c-axis oriented ZSM-5 crystals were successfully synthesized via a facile one-pot solvent-free route, using quartz fiber as silicon substrate and NH4HCO3 as the growing inhibitor on the crystal faces. The immigration of silica inside the quartz fibers formed the hollow morphology and the shell of hollow fiber was composed by the ZSM-5 crystals. In addition, the length of c-axis of ZSM-5 could be controlled by the amount of NH4HCO3, which selectively inhibited the growth on (010) surface. The obtained ZSM-5 hollow fibers gave a hierarchical structures composed by micro-, meso- and macropores. Catalytic tests for methanol to gasoline (MTG) revealed that the resultant ZSM-5 hollow fiber exhibited excellent performance with higher C5+ selectivity and longer lifetime due to the improved mass transfer inside the unique hollow fiber structure. |
| 关键词 | hollow fiber ZSM-5 solvent-free synthesis MTG heterogeneous catalysis |
| 收录类别 | SCI ; SCIE ; EI |
| 语种 | 英语 |
| 资助项目 | Strategic Priority Research Program of the Chinese Academy of Sciences[XDA21090204] |
| WOS研究方向 | Chemistry |
| WOS类目 | Chemistry, Physical |
| WOS记录号 | WOS:000455585000008 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| WOS关键词 | ENHANCED METHANOL ; ACID SITES ; ZEOLITE ; PERFORMANCE ; SAPO-34 ; FABRICATION ; ALKALINE |
| 原始文献类型 | Article |
| 引用统计 | 正在获取...
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| 文献类型 | 期刊论文 |
| 条目标识符 | https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/30164 |
| 专题 | 物质科学与技术学院_特聘教授组_孙予罕组 |
| 通讯作者 | Chen, Xinqing; Liu, Ziyu; Sun, Yuhan |
| 作者单位 | 1.Shanghai Univ, Sch Sci, Dept Chem, Shanghai 201900, Peoples R China 2.Chinese Acad Sci, Shanghai Adv Res Inst, CAS Key Lab Low Carbon Convers Sci & Engn, Shanghai 201210, Peoples R China 3.Univ Chinese Acad Sci, Beijing, Peoples R China 4.Shanghai Tech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China |
| 通讯作者单位 | 物质科学与技术学院 |
| 推荐引用方式 GB/T 7714 | Yu, Xing,Zhou, Cunhui,Chen, Xinqing,et al. Facile Solvent-free Synthesis of Hollow Fiber Catalyst Assembled by c-axis Oriented ZSM-5 Crystals[J]. CHEMCATCHEM,2018,10(24):5619-5626. |
| APA | Yu, Xing.,Zhou, Cunhui.,Chen, Xinqing.,Gao, Peng.,Qiu, Minghuang.,...&Sun, Yuhan.(2018).Facile Solvent-free Synthesis of Hollow Fiber Catalyst Assembled by c-axis Oriented ZSM-5 Crystals.CHEMCATCHEM,10(24),5619-5626. |
| MLA | Yu, Xing,et al."Facile Solvent-free Synthesis of Hollow Fiber Catalyst Assembled by c-axis Oriented ZSM-5 Crystals".CHEMCATCHEM 10.24(2018):5619-5626. |
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