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Surface Wrinkling with Memory for Programming Adhesion and Wettability
2023-03-24
发表期刊ACS APPLIED NANO MATERIALS (IF:5.3[JCR-2023],5.4[5-Year])
EISSN2574-0970
卷号6期号:6页码:4097-4104
发表状态已发表
DOI10.1021/acsanm.2c05410
摘要Modulating surface wrinkling is important for a variety of engineering applications. It has been known for more than two decades that the wavelength of surface wrinkles occurring in a metal film-soft polymer system scales linearly with the deposited film thickness. In the current experimental study of ultrathin gold film (0.2-8 nm) deposition on polydimethylsiloxane (PDMS), an unexplored thickness-dependent wrinkling phenomenon is found. By manipulating the deposition sequence as a degree of freedom for tailoring surface topography, we discovered a morphology memory effect where the wrinkle evolution in the subsequent deposition step inherits the surface pattern already formed in the previous step. Moreover, a stepwise deposition targeting 1 nm thick film can lead to 1 order of magnitude higher surface roughness than the one in the continuous deposition. By programming the sequences within 8 nm Au deposition, a surface strain map varying drastically from 0.2% to 27% is realized. Instructed by the strain map, we show the great potentials of tailored wrinkles in alternating surface wettability, enhancing surface Raman scattering, and on-demand tuning of surface adhesion. © 2023 The Authors. Published by American Chemical Society.
关键词Adhesion Degrees of freedom (mechanics) Deposition Metallic films Polydimethylsiloxane Raman scattering Silicones Surface roughness Surface scattering Topography Engineering applications Memory effects Metal-films Morphology memory effect Soft polymers Stepwise deposition Strain maps Surface adhesion Surface wrinkling Wrinkle
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收录类别EI ; SCI
语种英语
资助项目FRIPRO project Towards Design of Super-Low Ice Adhesion Surfaces[250990] ; PETROMAKS project Durable Arctic Icephobic Materials (AIM)["255507","245963/F50","302348"]
WOS研究方向Science & Technology - Other Topics ; Materials Science
WOS类目Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号WOS:000953971200001
出版者American Chemical Society
EI入藏号20231113741476
EI主题词Thick films
EI分类号741.1 Light/Optics ; 802.3 Chemical Operations ; 815.1.1 Organic Polymers ; 931 Classical Physics ; Quantum Theory ; Relativity ; 931.1 Mechanics ; 931.2 Physical Properties of Gases, Liquids and Solids ; 951 Materials Science
原始文献类型Journal article (JA)
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文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/290032
专题物质科学与技术学院
物质科学与技术学院_博士生
通讯作者He, Jianying; Zhang, Zhiliang
作者单位
1.Norwegian Univ Sci & Technol NTNU, Dept Struct Engn, N-7491 Trondheim, Norway
2.Foshan Southern China Inst New Mat, Foshan 528231, Peoples R China
3.Shenzhen Adventure Tech Co Ltd, Shenzhen 518000, Peoples R China
4.Norwegian Univ Sci & Technol NTNU, Dept Chem, N-7491 Trondheim, Norway
5.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
6.Chinese Acad Sci, Ctr Mat Synthet Biol, Shenzhen Inst Synthet Biol, Shenzhen 518055, Peoples R China
7.Chinese Acad Sci, CAS Key Lab Quantitat Engn Biol, Shenzhen Inst Synthet Biol, Shenzhen Inst Adv Technol, Shenzhen 518055, Peoples R China
推荐引用方式
GB/T 7714
Wang, Feng,Xiao, Senbo,Luo, Sihai,et al. Surface Wrinkling with Memory for Programming Adhesion and Wettability[J]. ACS APPLIED NANO MATERIALS,2023,6(6):4097-4104.
APA Wang, Feng.,Xiao, Senbo.,Luo, Sihai.,Fu, Yuequn.,Skallerud, Bjorn Helge.,...&Zhang, Zhiliang.(2023).Surface Wrinkling with Memory for Programming Adhesion and Wettability.ACS APPLIED NANO MATERIALS,6(6),4097-4104.
MLA Wang, Feng,et al."Surface Wrinkling with Memory for Programming Adhesion and Wettability".ACS APPLIED NANO MATERIALS 6.6(2023):4097-4104.
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