Generation of Raman lasers from nitrogen molecular ions driven by ultraintense laser fields
2018-03-29
发表期刊NEW JOURNAL OF PHYSICS
ISSN1367-2630
卷号20期号:3
发表状态已发表
DOI10.1088/1367-2630/aab087
摘要Atmospheric lasing has aroused much interest in the past few years. The 'air-laser' opens promising potential for remote chemical sensing of trace gases with high sensitivity and specificity. At present, several approaches have been successfully implemented for generating highly coherent laser beams in atmospheric condition, including both amplified-spontaneous emission, and narrow-bandwidth stimulated emission in the forward direction in the presence of self-generated or externally injected seed pulses. Here, we report on generation of multiple-wavelength Raman lasers from nitrogen molecular ions (N-2(+)), driven by intense mid-infrared laser fields. Intuitively, the approach appears problematic for the small nonlinear susceptibility of N-2(+) ions, whereas the efficiency of Raman laser can be significantly promoted in near-resonant condition. More surprisingly, a Raman laser consisting of a supercontinuum spanning from similar to 310 to similar to 392 nm has been observed resulting from a series near-resonant nonlinear processes including four-wave mixing, stimulated Raman scattering and cross phase modulation. To date, extreme nonlinear optics in molecular ions remains largely unexplored, which provides an alternative means for air-laser-based remote sensing applications.
关键词strong field physics supercontinuum generation tunnel ionization
收录类别SCI ; SCIE ; EI
语种英语
资助项目Shanghai Rising-Star Program[17QA1404600]
WOS研究方向Physics
WOS类目Physics, Multidisciplinary
WOS记录号WOS:000428905500010
出版者IOP PUBLISHING LTD
EI入藏号20181504991002
EI主题词Atmospheric chemistry ; Chemical sensors ; Four wave mixing ; Ion sources ; Ionization of gases ; Laser beams ; Nitrogen ; Optical parametric oscillators ; Pumping (laser) ; Remote sensing ; Supercontinuum generation
EI分类号Nonlinear Optics:741.1.1 ; Lasers, General:744.1 ; Laser Beam Interactions:744.8 ; Chemistry:801 ; Chemistry, General:801.1 ; Chemical Reactions:802.2 ; Chemical Products Generally:804 ; High Energy Physics:932.1
WOS关键词RARE-GASES ; AIR ; IONIZATION
原始文献类型Article
引用统计
文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/20224
专题物质科学与技术学院
物质科学与技术学院_特聘教授组_程亚组
物质科学与技术学院_博士生
通讯作者Cheng, Ya
作者单位
1.Chinese Acad Sci, Shanghai Inst Opt & Fine Mech, State Key Lab High Field Laser Phys, Shanghai 201800, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 200031, Peoples R China
4.East China Normal Univ, State Key Lab Precis Spect, Shanghai 200062, Peoples R China
5.Shanxi Univ, Collaborat Innovat Ctr Extreme Opt, Taiyuan 030006, Shanxi, Peoples R China
推荐引用方式
GB/T 7714
Yao, Jinping,Chu, Wei,Liu, Zhaoxiang,et al. Generation of Raman lasers from nitrogen molecular ions driven by ultraintense laser fields[J]. NEW JOURNAL OF PHYSICS,2018,20(3).
APA Yao, Jinping,Chu, Wei,Liu, Zhaoxiang,Xu, Bo,Chen, Jinming,&Cheng, Ya.(2018).Generation of Raman lasers from nitrogen molecular ions driven by ultraintense laser fields.NEW JOURNAL OF PHYSICS,20(3).
MLA Yao, Jinping,et al."Generation of Raman lasers from nitrogen molecular ions driven by ultraintense laser fields".NEW JOURNAL OF PHYSICS 20.3(2018).
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