A novel atmospheric tritium sampling system
2018-06
发表期刊NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT (IF:1.5[JCR-2023],1.4[5-Year])
ISSN0168-9002
卷号892页码:127-133
发表状态已发表
DOI10.1016/j.nima.2017.12.029
摘要The health hazard of tritium is related to its chemical form. Sampling different chemical forms of tritium simultaneously becomes significant. Here a novel atmospheric tritium sampling system (TS-212) was developed to collect the tritiated water (HTO), tritiated hydrogen (HT) and tritiated methane (CH3T) simultaneously. It consisted of an air inlet system, three parallel connected sampling channels, a hydrogen supply module, a methane supply module and a remote control system. It worked at air flow rate of 1 L/min to 5 L/min, with temperature of catalyst furnace at 200 degrees C for HT sampling and 400 degrees C for CH3T sampling. Conversion rates of both HT and CH3T to HTO were larger than 99%. The collecting efficiency of the two-stage trap sets for HTO was larger than 96% in 12 h working-time without being blocked. Therefore, the collected efficiencies of TS-212 are larger than 95% for tritium with different chemical forms in environment. Besides, the remote control system made sampling more intelligent, reducing the operator's work intensity. Based on the performance parameters described above, the TS-212 can be used to sample atmospheric tritium in different chemical forms. (C) 2017 Elsevier B.V. All rights reserved.
关键词Atmospheric tritium HTO HT CH3T Hydrogen supply module Methane supply module
收录类别SCI ; SCIE ; EI
语种英语
WOS研究方向Instruments & Instrumentation ; Nuclear Science & Technology ; Physics
WOS类目Instruments & Instrumentation ; Nuclear Science & Technology ; Physics, Nuclear ; Physics, Particles & Fields
WOS记录号WOS:000428924800016
出版者ELSEVIER SCIENCE BV
EI入藏号20181204934080
EI主题词Chemical hazards ; Collector efficiency ; Control systems ; Efficiency ; Health hazards ; Methane ; Remote control ; Tritium
EI分类号Atmospheric Properties:443.1 ; Health Care:461.7 ; Radioisotopes:622.1.1 ; Solar Cells:702.3 ; Control Systems:731.1 ; Organic Compounds:804.1 ; Production Engineering:913.1 ; Accidents and Accident Prevention:914.1
WOS关键词ENVIRONMENTAL TRITIUM ; REPROCESSING PLANT ; HYDROGEN ; JAPAN
原始文献类型Article
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文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/18240
专题物质科学与技术学院
物质科学与技术学院_博士生
通讯作者Liu, Wei; Liu, Guimin
作者单位
1.Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.CNNC Nucl Power Operat Management Co Ltd, Haiyan 314300, Peoples R China
4.ShanghaiTech Univ, Shanghai 200031, Peoples R China
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GB/T 7714
Qin, Lailai,Xia, Zhenghai,Gu, Shaozhong,et al. A novel atmospheric tritium sampling system[J]. NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT,2018,892:127-133.
APA Qin, Lailai.,Xia, Zhenghai.,Gu, Shaozhong.,Zhang, Dongxun.,Bao, Guangliang.,...&Liu, Guimin.(2018).A novel atmospheric tritium sampling system.NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT,892,127-133.
MLA Qin, Lailai,et al."A novel atmospheric tritium sampling system".NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT 892(2018):127-133.
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