"Burr Puzzle"-Like Hierarchical Beta zeolite composed of crisscrossed nanorods

doi:10.1016/j.micromeso.2022.111843

	"Burr Puzzle"-Like Hierarchical Beta zeolite composed of crisscrossed nanorods
	Li, Shiqing 1; Si, Xiaomeng2 ; Peng, Rusi 1; Pan, Huang 1; Xu, Hao 1; Jiang, Jingang 1; Ma, Yanhang2,3 ; Wu, Peng 1,4
	2022-04
发表期刊	MICROPOROUS AND MESOPOROUS MATERIALS (IF:4.8[JCR-2023],4.7[5-Year])
ISSN	1387-1811
EISSN	1873-3093
卷号	335
发表状态	已发表
DOI	10.1016/j.micromeso.2022.111843
摘要	Hierarchical Beta zeolite (named ECNU-41) was directly synthesized with commercially available ionic liquid 1-butyl-1-methylpyrrolidinium hydroxide as organic structure-directing agent (OSDA) in the absence of any surfactants or polymers. The ECNU-41 crystals were composed of nanorods through a unique stacking manner, exhibiting a morphology resembling the Chinese traditional toy "burr puzzle". The orderly crisscrossed stacking ECNU-41 possesses high hydrothermal stability, abundant intercrystal mesoporosity, and enriched phase of polymorph B. In comparison to conventional nanosized Beta zeolites, ECNU-41 aluminosilicate and titanosilicate exhibited more remarkable and competitive catalytic performances in a variety of reactions, including benzene alkylation, methanol to propylene, and alkenes epoxidation. With improved diffusion rate and mass transfer due to the hierarchical structure, ECNU-41 is expected to serve as promising catalysts for those reactions involving bulky molecules. © 2022 Elsevier Inc.
关键词	Alkylation Benzene Ionic liquids Mass transfer Nanorods Olefins Organic polymers Toys Alkenes epoxidations Benzene alkylation Beta zeolite Hierarchical pores MTP reaction Organic structures Stackings Structure directing agents Synthesised Zeolite beta
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收录类别	SCI ; SCIE ; EI
语种	英语
资助项目	NSFC of China[21872052,21972043,21972044] ; China Ministry of Science and Technology[2021YFA1501401] ; Shanghai Science and Technology Plan[21DZ2260400] ; National Key Research and Development Program of China and ChEM[21835002] ; SPST of Shanghai Tech University[EM02161943]
WOS研究方向	Chemistry ; Science & Technology - Other Topics ; Materials Science
WOS类目	Chemistry, Applied ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号	WOS:000791315000002
出版者	Elsevier B.V.
EI入藏号	20221311867772
EI主题词	Zeolites
EI分类号	641.3 Mass Transfer ; 761 Nanotechnology ; 802.2 Chemical Reactions ; 804 Chemical Products Generally ; 804.1 Organic Compounds ; 804.2 Inorganic Compounds ; 815.1.1 Organic Polymers ; 933 Solid State Physics
原始文献类型	Journal article (JA)
引用统计	正在获取...
文献类型	期刊论文
条目标识符	https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/169304
专题	物质科学与技术学院_博士生物质科学与技术学院_PI研究组_马延航组
共同第一作者	Si, Xiaomeng
通讯作者	Xu, Hao; Jiang, Jingang; Wu, Peng
作者单位	1.East China Normal Univ, Sch Chem & Mol Engn, Shanghai Key Lab Green Chem & Chem Proc, North Zhongshan Rd 3663, Shanghai 200062, Peoples R China 2.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China 3.ShanghaiTech Univ, Shanghai Key Lab High resolut Electron Microscopy, Shanghai 201210, Peoples R China 4.Inst Ecochongming, Shanghai 202162, Peoples R China
推荐引用方式 GB/T 7714	Li, Shiqing,Si, Xiaomeng,Peng, Rusi,et al. "Burr Puzzle"-Like Hierarchical Beta zeolite composed of crisscrossed nanorods[J]. MICROPOROUS AND MESOPOROUS MATERIALS,2022,335.
APA	Li, Shiqing.,Si, Xiaomeng.,Peng, Rusi.,Pan, Huang.,Xu, Hao.,...&Wu, Peng.(2022)."Burr Puzzle"-Like Hierarchical Beta zeolite composed of crisscrossed nanorods.MICROPOROUS AND MESOPOROUS MATERIALS,335.
MLA	Li, Shiqing,et al.""Burr Puzzle"-Like Hierarchical Beta zeolite composed of crisscrossed nanorods".MICROPOROUS AND MESOPOROUS MATERIALS 335(2022).