Melting-assisted solvent-free synthesis of hierarchical SAPO-34 with enhanced methanol to olefins (MTO) performance
2018-01-21
发表期刊CATALYSIS SCIENCE & TECHNOLOGY
ISSN2044-4753
卷号8期号:2页码:423-427
发表状态已发表
DOI10.1039/c7cy02283b
摘要SAPO-34 zeolite with a butterfly patterned hierarchical pore system and high relative crystallinity was synthesized by a melting-assisted solvent-free route. Oxalic acid in the solid state was used as the etching agent through a facile thermal treatment of the parent SAPO-34. The resultant zeolite exhibited complete methanol conversion, high C-2(=)-C-4(=) selectivity (> 91%) and a long lifetime in the MTO process.
收录类别SCI ; SCIE ; EI
语种英语
资助项目Science and Technology Commission of Shanghai Municipality[14DZ1207602] ; Science and Technology Commission of Shanghai Municipality[16DZ1206900]
WOS研究方向Chemistry
WOS类目Chemistry, Physical
WOS记录号WOS:000423483200002
出版者ROYAL SOC CHEMISTRY
EI入藏号20180504699413
EI主题词Melting ; Methanol ; Oxalic acid ; Zeolites
EI分类号Chemical Operations:802.3 ; Organic Compounds:804.1 ; Inorganic Compounds:804.2
WOS关键词CATALYTIC-ACTIVITY ; MOLECULAR-SIEVES ; ZEOLITES ; SILICOALUMINOPHOSPHATES ; SPECTROSCOPY ; SELECTIVITY ; CONVERSION ; H-SAPO-34 ; CRYSTALS
原始文献类型Article
引用统计
文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/16298
专题物质科学与技术学院
物质科学与技术学院_特聘教授组_孙予罕组
物质科学与技术学院_硕士生
通讯作者Chen, Xinqing; Sun, Yuhan
作者单位
1.Chinese Acad Sci, Adv Res Inst, CAS Key Lab Low Carbon Convers Sci & Engn, Shanghai, Peoples R China
2.Shanghai Tech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
3.Shanghai Univ, Shanghai 200444, Peoples R China
4.Sinopec Shanghai Res Inst Petrochem Technol, Shanghai, Peoples R China
通讯作者单位物质科学与技术学院
推荐引用方式
GB/T 7714
Liu, Ziyu,Ren, Shu,Yu, Xing,et al. Melting-assisted solvent-free synthesis of hierarchical SAPO-34 with enhanced methanol to olefins (MTO) performance[J]. CATALYSIS SCIENCE & TECHNOLOGY,2018,8(2):423-427.
APA Liu, Ziyu.,Ren, Shu.,Yu, Xing.,Chen, Xinqing.,Wang, Gang.,...&Sun, Yuhan.(2018).Melting-assisted solvent-free synthesis of hierarchical SAPO-34 with enhanced methanol to olefins (MTO) performance.CATALYSIS SCIENCE & TECHNOLOGY,8(2),423-427.
MLA Liu, Ziyu,et al."Melting-assisted solvent-free synthesis of hierarchical SAPO-34 with enhanced methanol to olefins (MTO) performance".CATALYSIS SCIENCE & TECHNOLOGY 8.2(2018):423-427.
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