Background-free single-beam coherent Raman spectroscopy assisted by air lasing
2022-02-01
发表期刊OPTICS LETTERS (IF:3.1[JCR-2023],3.1[5-Year])
ISSN0146-9592
EISSN1539-4794
卷号47期号:3页码:481-484
发表状态已发表
DOI10.1364/OL.441602
摘要

We develop a background-free single-beam coherent Raman scattering technique enabling the high-sensitivity detection of greenhouse gases. In this scheme, Raman coherence prepared by a femtosecond laser is interrogated by self-generated narrowband air lasing, thus allowing single-beam measurements without complex pulse shaping. The unique temporal and spectral characteristics of air lasing are beneficial for improving the signal-to-noise ratio and spectral resolution of Raman signals. With this method, SF6 gas present at a concentration of 0.38% was detected in an SF6-air mixture. This technique provides a simple and promising route for remote detection due to the low divergence of Raman signals and the availability of high-energy pump lasers, which may broaden the potential applications of air lasing. © 2022 Optical Society of America

关键词Coherent scattering Greenhouse gases Pulse shaping Pumping (laser) Signal to noise ratio Sulfur hexafluoride Beam measurements Coherent Raman scattering Greenhouses gas High-sensitivity detection Lasings Narrow bands Raman coherence Raman signal Scattering techniques Single-beam
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收录类别SCI ; SCIE ; EI
语种英语
资助项目National Natural Science Foundation of China[11822410,12034013,12064009,12074063] ; Key Research Program of Frontier Sciences of Chinese Academy of Sciences[QYZDJ-SSW-SLH010] ; Program of Shanghai Academic Research Leader[20XD1424200] ; Shanghai Municipal Science and Technology Major Project[2019SHZDZX01] ; Youth Innovation Promotion Association of the Chinese Academy of Sciences[2018284]
WOS研究方向Optics
WOS类目Optics
WOS记录号WOS:000749682500010
出版者The Optical Society
EI入藏号20220411531199
EI主题词Raman spectroscopy
EI分类号451.1 Air Pollution Sources ; 711 Electromagnetic Waves ; 713.4 Pulse Circuits ; 716.1 Information Theory and Signal Processing ; 744.1 Lasers, General ; 804.2 Inorganic Compounds
原始文献类型Journal article (JA)
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文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/153595
专题物质科学与技术学院_博士生
通讯作者Yao, Jinping
作者单位
1.Chinese Acad Sci, Shanghai Inst Opt & Fine Mech, State Key Lab High Field Laser Phys, Shanghai 201800, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.East China Univ Technol, Sch Sci, Nanchang 330013, Jiangxi, Peoples R China
4.Shanghai Jiao Tong Univ, Sch Phys & Astron, Shanghai 200240, Peoples R China
5.Shanghai Tech Univ, Sch Phys Sci & Technol, Shanghai 200031, Peoples R China
6.East China Jiaotong Univ, Sch Sci, Nanchang 330013, Jiangxi, Peoples R China
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GB/T 7714
Zhang, Fangbo,Xie, Hongqiang,Yuan, Luqi,et al. Background-free single-beam coherent Raman spectroscopy assisted by air lasing[J]. OPTICS LETTERS,2022,47(3):481-484.
APA Zhang, Fangbo.,Xie, Hongqiang.,Yuan, Luqi.,Zhang, Zhihao.,Fu, Botao.,...&Xu, Zhizhan.(2022).Background-free single-beam coherent Raman spectroscopy assisted by air lasing.OPTICS LETTERS,47(3),481-484.
MLA Zhang, Fangbo,et al."Background-free single-beam coherent Raman spectroscopy assisted by air lasing".OPTICS LETTERS 47.3(2022):481-484.
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