ShanghaiTech University Knowledge Management System
| Application of Electron-Rich Covalent Organic Frameworks COF-JLU25 for Photocatalytic Aerobic Oxidative Hydroxylation of Arylboronic Acids to Phenols | |
| 2021-08-06 | |
| 发表期刊 | EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
 |
| ISSN | 1434-193X |
| EISSN | 1099-0690 |
| 卷号 | 2021期号:29页码:3986-3991 |
| 发表状态 | 已发表 |
| DOI | 10.1002/ejoc.202100173 |
| 摘要 | Visible-light-driven organic reactions are environmentally friendly green chemical transformations among which photosynthetic oxidative hydroxylation of arylboronic acids to phenols has attracted increasing research interest during the very recent years. Given the efficiency and reusability of heterogeneous catalysts, COF-JLU25, an electron-rich COF-based photocatalyst constructed by integrating electron-donating blocks 1,3,6,8-tetrakis(4-aminophenyl)pyrene (PyTA) and 4-[4-(4-formylmethyl)-2,5-dimethoxyphenyl] benzaldehyde (TpDA), was selected as a photocatalyst for the oxidative hydroxylation of arylboronic acids. In our studies, COF-JLU25 demonstrated excellent photocatalytic activity with high efficiency, robust reusability, and low catalyst loading, showcasing an application potential of previously underexplored COF-based photocatalyst composed solely of electron-rich units. |
| 关键词 | Arylboronic acids Covalent organic frameworks Oxidative hydroxylation Photocatalysis Superoxide radical |
| 收录类别 | SCIE |
| 语种 | 英语 |
| WOS研究方向 | Chemistry |
| WOS类目 | Chemistry, Organic |
| WOS记录号 | WOS:000632317800001 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 原始文献类型 | Article |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 条目标识符 | https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/126153 |
| 专题 | 物质科学与技术学院_硕士生 物质科学与技术学院_特聘教授组_杨辉组 物质科学与技术学院_特聘教授组_文珂组 |
| 通讯作者 | Wen, Ke |
| 作者单位 | 1.Chinese Acad Sci Shanghai, Shanghai Adv Res Inst, Shanghai, Peoples R China; 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China; 3.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China; 4.ChemBridge Res Labs, Med Chem, San Diego, CA 92127 USA |
| 第一作者单位 | 物质科学与技术学院 |
| 通讯作者单位 | 物质科学与技术学院 |
| 推荐引用方式 GB/T 7714 | Xiao, Guangju,Li, Wenqian,Chen, Tao,et al. Application of Electron-Rich Covalent Organic Frameworks COF-JLU25 for Photocatalytic Aerobic Oxidative Hydroxylation of Arylboronic Acids to Phenols[J]. EUROPEAN JOURNAL OF ORGANIC CHEMISTRY,2021,2021(29):3986-3991. |
| APA | Xiao, Guangju.,Li, Wenqian.,Chen, Tao.,Hu, Wei-Bo.,Yang, Hui.,...&Wen, Ke.(2021).Application of Electron-Rich Covalent Organic Frameworks COF-JLU25 for Photocatalytic Aerobic Oxidative Hydroxylation of Arylboronic Acids to Phenols.EUROPEAN JOURNAL OF ORGANIC CHEMISTRY,2021(29),3986-3991. |
| MLA | Xiao, Guangju,et al."Application of Electron-Rich Covalent Organic Frameworks COF-JLU25 for Photocatalytic Aerobic Oxidative Hydroxylation of Arylboronic Acids to Phenols".EUROPEAN JOURNAL OF ORGANIC CHEMISTRY 2021.29(2021):3986-3991. |
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