Single-atom catalysts for metal-sulfur batteries: Current progress and future perspectives

doi:10.1016/j.jechem.2020.06.018

	Single-atom catalysts for metal-sulfur batteries: Current progress and future perspectives
	Xiao, Ru 1,2; Chen, Ke1,3 ; Zhang, Xiaoyin 1,2; Yang, Zhenzhen 1,5; Hu, Guangjian 1,2; Sun, Zhenhua 1,2; Cheng, Hui-Ming 1,2,4; Li, Feng 1,2
	2021-03
发表期刊	JOURNAL OF ENERGY CHEMISTRY (IF:14.0[JCR-2023],12.3[5-Year])
ISSN	2095-4956
卷号	54 页码:452-466
发表状态	已发表
DOI	10.1016/j.jechem.2020.06.018
摘要	Metal-sulfur batteries are recognized as a promising candidate for next generation electrochemical energy storage systems owing to their high theoretical energy density, low cost and environmental friendliness. However, sluggish redox kinetics of sulfur species and the shuttle effect lead to large polarization and severe capacity decay. Numerous approaches from physical barrier, chemical adsorption strategies to electrocatalysts have been tried to solve these issues and pushed the rate and cycle performance of sulfur electrodes to higher levels. Most recently, single-atom catalysts (SACs) with high catalytic efficiency have been introduced into metal-sulfur systems to achieve fast redox kinetics of sulfur conversion. In this review, we systematically summarize the current progress on SACs for sulfur electrodes from aspects of synthesis, characterization and electrochemical performance. Challenges and potential solutions for designing SACs for high-performance sulfur electrodes are discussed. © 2020 Science Press
关键词	Single-atom catalysts Metal-sulfur batteries Redox kinetics Synthesis Characterization Electrochemical performance
收录类别	SCI ; SCIE ; EI
资助项目	National Natural Science Foundation of China[51972313][51525206][51927803] ; Ministry of Science and Technology of China[2016YFA0200100][2016YFB0100100] ; Strategic Priority Research Program of Chinese Academy of Science[XDA22010602] ; Youth Innovation Promotion Association of the Chinese Academy of Sciences[Y201942] ; Key Research Program of Chinese Academy of Sciences[KGZD-EW-T06] ; Special Projects of the Central Government in Guidance of Local Science and Technology Development[2020JH6/10500024] ; China Petrochemical Cooperation[218025] ; Economic, The Bureau of Industry and Information Technology of Shenzhen for the
WOS研究方向	Chemistry ; Energy & Fuels ; Engineering
WOS类目	Chemistry, Applied ; Chemistry, Physical ; Energy & Fuels ; Engineering, Chemical
WOS记录号	WOS:000605249800011
出版者	Elsevier B.V.
EI入藏号	20202808915759
EI主题词	Electric batteries ; Electrocatalysts ; Electrochemical electrodes
EI分类号	Electric Batteries:702.1 ; Chemical Agents and Basic Industrial Chemicals:803 ; Chemical Products Generally:804
原始文献类型	Journal article (JA)
引用统计	正在获取...
文献类型	期刊论文
条目标识符	https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/122663
专题	物质科学与技术学院_博士生
通讯作者	Sun, Zhenhua; Li, Feng
作者单位	1.Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang; Liaoning; 110016, China 2.School of Materials Science and Engineering, University of Science and Technology of China, Hefei; Anhui; 230026, China 3.School of Physical Science and Technology, ShanghaiTech University, Shanghai; 201210, China 4.Shenzhen Geim Graphene Center, Tsinghua-Berkeley Shenzhen Institute, Tsinghua University, Shenzhen; Guangdong; 518055, China 5.Key Laboratory of Physics and Technology for Advanced Batteries (Ministry of Education), College of Physics, Jilin University, Changchun; Jilin; 130012, China
推荐引用方式 GB/T 7714	Xiao, Ru,Chen, Ke,Zhang, Xiaoyin,et al. Single-atom catalysts for metal-sulfur batteries: Current progress and future perspectives[J]. JOURNAL OF ENERGY CHEMISTRY,2021,54:452-466.
APA	Xiao, Ru.,Chen, Ke.,Zhang, Xiaoyin.,Yang, Zhenzhen.,Hu, Guangjian.,...&Li, Feng.(2021).Single-atom catalysts for metal-sulfur batteries: Current progress and future perspectives.JOURNAL OF ENERGY CHEMISTRY,54,452-466.
MLA	Xiao, Ru,et al."Single-atom catalysts for metal-sulfur batteries: Current progress and future perspectives".JOURNAL OF ENERGY CHEMISTRY 54(2021):452-466.