Non-Coulomb strong electron-hole binding in Ta2NiSe5 revealed by time- and angle-resolved photoemission spectroscopy
2020-06-22
发表期刊PHYSICAL REVIEW B (IF:3.2[JCR-2023],3.3[5-Year])
ISSN2469-9950
EISSN2469-9969
卷号101期号:23
发表状态已发表
DOI10.1103/PhysRevB.101.235148
摘要We reveal an ultrafast purely electronic phase transition in Ta2NiSe5, which is a plausible excitonic insulator, after excited by an ultrafast infrared laser pulse. Specifically, the order parameter of the strong electron-hole binding shrinks with enhancing the pump pulse, and above a critical pump fluence, a photoexcited semimetallic state is experimentally identified with the absence of ultrafast structural transition. In addition, the bare valence and conduction bands and also the effective masses in Ta2NiSe5 are determined. These findings and detailed analysis suggest a bare nonequilibrium semimetallic phase in Ta2NiSe5 and the strong electron-hole binding cannot be exclusively driven by Coulomb interaction.
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收录类别SCI ; SCIE ; EI
语种英语
资助项目Ministry of Science and Technology of China[2016YFA0301003][2016YFA0300501] ; National Natural Science Foundation of China[11874264][11674224][11974243][11704247][U1632272][11521404] ; Natural Science Foundation of Shanghai[17ZR1443300]
WOS研究方向Materials Science ; Physics
WOS类目Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS记录号WOS:000541702100002
出版者AMER PHYSICAL SOC
WOS关键词PHASE
原始文献类型Article
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文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/121860
专题物质科学与技术学院_博士生
物质科学与技术学院_PI研究组_郭艳峰组
通讯作者Zhang, Wentao
作者单位
1.Shanghai Jiao Tong Univ, Sch Phys & Astron, Key Lab Artificial Struct & Quantum Control, Minist Educ,Shenyang Natl Lab Mat Sci, Shanghai 200240, Peoples R China
2.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
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Tang, Tianwei,Wang, Hongyuan,Duan, Shafeng,et al. Non-Coulomb strong electron-hole binding in Ta2NiSe5 revealed by time- and angle-resolved photoemission spectroscopy[J]. PHYSICAL REVIEW B,2020,101(23).
APA Tang, Tianwei.,Wang, Hongyuan.,Duan, Shafeng.,Yang, Yuanyuan.,Huang, Chaozhi.,...&Zhang, Wentao.(2020).Non-Coulomb strong electron-hole binding in Ta2NiSe5 revealed by time- and angle-resolved photoemission spectroscopy.PHYSICAL REVIEW B,101(23).
MLA Tang, Tianwei,et al."Non-Coulomb strong electron-hole binding in Ta2NiSe5 revealed by time- and angle-resolved photoemission spectroscopy".PHYSICAL REVIEW B 101.23(2020).
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