Melting-assisted solvent-free synthesis of hierarchical SAPO-34 with enhanced methanol to olefins (MTO) performance

doi:10.1039/c7cy02283b

	Melting-assisted solvent-free synthesis of hierarchical SAPO-34 with enhanced methanol to olefins (MTO) performance
	Liu, Ziyu 1; Ren, Shu 1,4; Yu, Xing 1,3; Chen, Xinqing 1; Wang, Gang 1; Wu, Xian 1,3; Yu, Gan1,2 ; Qiu, Minghuang 1; Yang, Chengguang 1; Sun, Yuhan1,2
	2018-01-21
发表期刊	CATALYSIS SCIENCE & TECHNOLOGY
ISSN	2044-4753
卷号	8 期号:2 页码:423-427
发表状态	已发表
DOI	10.1039/c7cy02283b
摘要	SAPO-34 zeolite with a butterfly patterned hierarchical pore system and high relative crystallinity was synthesized by a melting-assisted solvent-free route. Oxalic acid in the solid state was used as the etching agent through a facile thermal treatment of the parent SAPO-34. The resultant zeolite exhibited complete methanol conversion, high C-2(=)-C-4(=) selectivity (> 91%) and a long lifetime in the MTO process.
收录类别	SCI ; SCIE ; EI
语种	英语
资助项目	Science and Technology Commission of Shanghai Municipality[14DZ1207602] ; Science and Technology Commission of Shanghai Municipality[16DZ1206900]
WOS研究方向	Chemistry
WOS类目	Chemistry, Physical
WOS记录号	WOS:000423483200002
出版者	ROYAL SOC CHEMISTRY
EI入藏号	20180504699413
EI主题词	Melting ; Methanol ; Oxalic acid ; Zeolites
EI分类号	Chemical Operations:802.3 ; Organic Compounds:804.1 ; Inorganic Compounds:804.2
WOS关键词	CATALYTIC-ACTIVITY ; MOLECULAR-SIEVES ; ZEOLITES ; SILICOALUMINOPHOSPHATES ; SPECTROSCOPY ; SELECTIVITY ; CONVERSION ; H-SAPO-34 ; CRYSTALS
原始文献类型	Article
引用统计
文献类型	期刊论文
条目标识符	https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/16298
专题	物质科学与技术学院物质科学与技术学院_特聘教授组_孙予罕组物质科学与技术学院_硕士生
通讯作者	Chen, Xinqing; Sun, Yuhan
作者单位	1.Chinese Acad Sci, Adv Res Inst, CAS Key Lab Low Carbon Convers Sci & Engn, Shanghai, Peoples R China 2.Shanghai Tech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China 3.Shanghai Univ, Shanghai 200444, Peoples R China 4.Sinopec Shanghai Res Inst Petrochem Technol, Shanghai, Peoples R China
通讯作者单位	物质科学与技术学院
推荐引用方式 GB/T 7714	Liu, Ziyu,Ren, Shu,Yu, Xing,et al. Melting-assisted solvent-free synthesis of hierarchical SAPO-34 with enhanced methanol to olefins (MTO) performance[J]. CATALYSIS SCIENCE & TECHNOLOGY,2018,8(2):423-427.
APA	Liu, Ziyu.,Ren, Shu.,Yu, Xing.,Chen, Xinqing.,Wang, Gang.,...&Sun, Yuhan.(2018).Melting-assisted solvent-free synthesis of hierarchical SAPO-34 with enhanced methanol to olefins (MTO) performance.CATALYSIS SCIENCE & TECHNOLOGY,8(2),423-427.
MLA	Liu, Ziyu,et al."Melting-assisted solvent-free synthesis of hierarchical SAPO-34 with enhanced methanol to olefins (MTO) performance".CATALYSIS SCIENCE & TECHNOLOGY 8.2(2018):423-427.