Engineering of Pore Geometry for Ultrahigh Capacity Methane Storage in Mesoporous Metal-Organic Frameworks
Liang, Cong-Cong1; Shi, Zhao-Lin1; He, Chun-Ting2; Tan, Jing1; Zhou, Hu-Die1; Zhou, Hao-Long1; Lee, Yongjin1; Zhang, Yue-Biao1
2017-09-27
Source PublicationJOURNAL OF THE AMERICAN CHEMICAL SOCIETY
ISSN0002-7863
Volume139Issue:38Pages:13300-13303
Status已发表
DOI10.1021/jacs.7b08347
Abstract

Mesoporous Zn4O(-COO)(6)-based metal organic frameworks (MOFs), including UMCM-1, MOF-205, MUF-7a, and the newly synthesized MOFs, termed ST-1, ST-2, ST-3, and ST-4 (ST = ShanghaiTech University), have been systematically investigated for ultra-high capacity methane storage. Exceptionally, ST-2 was found to have the highest deliverable capacity of 289 cm(3)srp/cm(3) (567 mg/g) at 298 K and 5-200 bar, which surpasses all previously reported records held by porous materials. We illustrate that the fine-tuned mesoporosity is critical in further improving the deliverable capacities at ultrahigh pressure.

Indexed BySCI ; EI
Funding ProjectNational Postdoctoral Program for Innovative Talents[BX201600195] ; National Postdoctoral Program for Innovative Talents[BX201700272]
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
WOS IDWOS:000412043000012
PublisherAMER CHEMICAL SOC
EI Accession Number20174004226756
EI KeywordsCrystalline materials ; Organometallics ; Porous materials
EI Classification NumberOrganic Compounds:804.1 ; Crystalline Solids:933.1 ; Materials Science:951
WOS KeywordNANOPOROUS MATERIALS ; WORKING CAPACITY ; NATURAL-GAS ; ADSORPTION ; CHEMISTRY ; POROSITY ; SITES ; MOFS
Original Document TypeArticle
Citation statistics
Cited Times:82[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttps://kms.shanghaitech.edu.cn/handle/2MSLDSTB/9906
Collection物质科学与技术学院
物质科学与技术学院_PI研究组_章跃标组
物质科学与技术学院_PI研究组_yongjin lee组
物质科学与技术学院_硕士生
物质科学与技术学院_本科生
物质科学与技术学院_博士生
Corresponding AuthorZhang, Yue-Biao
Affiliation1.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
2.Sun Yat Sen Univ, Sch Chem, Guangzhou 510275, Guangdong, Peoples R China
First Author AffilicationSchool of Physical Science and Technology
Corresponding Author AffilicationSchool of Physical Science and Technology
First Signature AffilicationSchool of Physical Science and Technology
Recommended Citation
GB/T 7714
Liang, Cong-Cong,Shi, Zhao-Lin,He, Chun-Ting,et al. Engineering of Pore Geometry for Ultrahigh Capacity Methane Storage in Mesoporous Metal-Organic Frameworks[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2017,139(38):13300-13303.
APA Liang, Cong-Cong.,Shi, Zhao-Lin.,He, Chun-Ting.,Tan, Jing.,Zhou, Hu-Die.,...&Zhang, Yue-Biao.(2017).Engineering of Pore Geometry for Ultrahigh Capacity Methane Storage in Mesoporous Metal-Organic Frameworks.JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,139(38),13300-13303.
MLA Liang, Cong-Cong,et al."Engineering of Pore Geometry for Ultrahigh Capacity Methane Storage in Mesoporous Metal-Organic Frameworks".JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 139.38(2017):13300-13303.
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