Engineering of Pore Geometry for Ultrahigh Capacity Methane Storage in Mesoporous Metal-Organic Frameworks

doi:10.1021/jacs.7b08347

	Engineering of Pore Geometry for Ultrahigh Capacity Methane Storage in Mesoporous Metal-Organic Frameworks
	Liang, Cong-Cong1 ; Shi, Zhao-Lin1 ; He, Chun-Ting 2; Tan, Jing1 ; Zhou, Hu-Die1 ; Zhou, Hao-Long1 ; Lee, Yongjin1 ; Zhang, Yue-Biao1
	2017-09-27
发表期刊	JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
ISSN	0002-7863
卷号	139 期号:38 页码:13300-13303
发表状态	已发表
DOI	10.1021/jacs.7b08347
摘要	Mesoporous Zn4O(-COO)(6)-based metal organic frameworks (MOFs), including UMCM-1, MOF-205, MUF-7a, and the newly synthesized MOFs, termed ST-1, ST-2, ST-3, and ST-4 (ST = ShanghaiTech University), have been systematically investigated for ultra-high capacity methane storage. Exceptionally, ST-2 was found to have the highest deliverable capacity of 289 cm(3)srp/cm(3) (567 mg/g) at 298 K and 5-200 bar, which surpasses all previously reported records held by porous materials. We illustrate that the fine-tuned mesoporosity is critical in further improving the deliverable capacities at ultrahigh pressure.
收录类别	SCI ; EI
资助项目	National Postdoctoral Program for Innovative Talents[BX201600195] ; National Postdoctoral Program for Innovative Talents[BX201700272]
WOS研究方向	Chemistry
WOS类目	Chemistry, Multidisciplinary
WOS记录号	WOS:000412043000012
出版者	AMER CHEMICAL SOC
EI入藏号	20174004226756
EI主题词	Crystalline materials ; Organometallics ; Porous materials
EI分类号	Organic Compounds:804.1 ; Crystalline Solids:933.1 ; Materials Science:951
WOS关键词	NANOPOROUS MATERIALS ; WORKING CAPACITY ; NATURAL-GAS ; ADSORPTION ; CHEMISTRY ; POROSITY ; SITES ; MOFS
原始文献类型	Article
引用统计
文献类型	期刊论文
条目标识符	https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/9906
专题	物质科学与技术学院物质科学与技术学院_PI研究组_章跃标组物质科学与技术学院_PI研究组_yongjin lee组物质科学与技术学院_硕士生物质科学与技术学院_本科生物质科学与技术学院_博士生
通讯作者	Zhang, Yue-Biao
作者单位	1.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China 2.Sun Yat Sen Univ, Sch Chem, Guangzhou 510275, Guangdong, Peoples R China
第一作者单位	物质科学与技术学院
通讯作者单位	物质科学与技术学院
第一作者的第一单位	物质科学与技术学院
推荐引用方式 GB/T 7714	Liang, Cong-Cong,Shi, Zhao-Lin,He, Chun-Ting,et al. Engineering of Pore Geometry for Ultrahigh Capacity Methane Storage in Mesoporous Metal-Organic Frameworks[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2017,139(38):13300-13303.
APA	Liang, Cong-Cong.,Shi, Zhao-Lin.,He, Chun-Ting.,Tan, Jing.,Zhou, Hu-Die.,...&Zhang, Yue-Biao.(2017).Engineering of Pore Geometry for Ultrahigh Capacity Methane Storage in Mesoporous Metal-Organic Frameworks.JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,139(38),13300-13303.
MLA	Liang, Cong-Cong,et al."Engineering of Pore Geometry for Ultrahigh Capacity Methane Storage in Mesoporous Metal-Organic Frameworks".JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 139.38(2017):13300-13303.