Microcavity Nonlinear Optics with an Organically Functionalized Surface
Chen, Jin-hui1; Shen, Xiaoqin2; Tang, Shui-Jing1,3,4,5; Cao, Qi-Tao1,3,4; Gong, Qihuang1,3,4,5,6; Xiao, Yun-Feng1,3,4,5,6
2019-10-24
Source PublicationPHYSICAL REVIEW LETTERS
ISSN0031-9007
Volume123Issue:17
DOI10.1103/PhysRevLett.123.173902
AbstractWe report enhanced optical nonlinear effects at the surface of an ultrahigh-Q silica microcavity functionalized by a thin layer of organic molecules. The maximal conversion efficiency of third harmonic generation reaches similar to 1680%/W-2 and an absolute efficiency of 0.0144% at pump power of similar to 2.90 mW, which is approximately 4 orders of magnitude higher than that in a reported silica microcavity. Further analysis clarifies the elusive dependence of the third harmonic signal on the pump power in previous literature. Molecule-functionalized microcavities may find promising applications in high-efficiency broadband optical frequency conversion and offer potential in sensitive surface analysis.
Indexed BySCI
Language英语
Funding ProjectChina Postdoctoral Science Foundation[2018M640015]
WOS Research AreaPhysics
WOS SubjectPhysics, Multidisciplinary
WOS IDWOS:000492373300004
PublisherAMER PHYSICAL SOC
EISSN1079-7114
WOS KeywordGENERATION ; RESONATOR ; EMISSION ; CHAOS
Original Document TypeArticle
Citation statistics
Cited Times [WOS]:0   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://kms.shanghaitech.edu.cn/handle/2MSLDSTB/80510
Collection物质科学与技术学院_PI研究组_沈晓钦组
Corresponding AuthorXiao, Yun-Feng
Affiliation1.Peking Univ, Sch Phys, State Key Lab Artificial Microstruct & Mesoscop P, Beijing 100871, Peoples R China
2.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
3.Frontiers Sci Ctr Nanooptoelect, Beijing 100871, Peoples R China
4.Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China
5.Shanxi Univ, Collaborat Innovat Ctr Extreme Opt, Taiyuan 030006, Shanxi, Peoples R China
6.Beijing Acad Quantum Informat Sci, Beijing 100193, Peoples R China
Recommended Citation
GB/T 7714
Chen, Jin-hui,Shen, Xiaoqin,Tang, Shui-Jing,et al. Microcavity Nonlinear Optics with an Organically Functionalized Surface[J]. PHYSICAL REVIEW LETTERS,2019,123(17).
APA Chen, Jin-hui,Shen, Xiaoqin,Tang, Shui-Jing,Cao, Qi-Tao,Gong, Qihuang,&Xiao, Yun-Feng.(2019).Microcavity Nonlinear Optics with an Organically Functionalized Surface.PHYSICAL REVIEW LETTERS,123(17).
MLA Chen, Jin-hui,et al."Microcavity Nonlinear Optics with an Organically Functionalized Surface".PHYSICAL REVIEW LETTERS 123.17(2019).
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