Microcavity Nonlinear Optics with an Organically Functionalized Surface

doi:10.1103/PhysRevLett.123.173902

	Microcavity Nonlinear Optics with an Organically Functionalized Surface
	Chen, Jin-hui 1; Shen, Xiaoqin2 ; Tang, Shui-Jing 1,3,4,5; Cao, Qi-Tao 1,3,4; Gong, Qihuang 1,3,4,5,6; Xiao, Yun-Feng 1,3,4,5,6
	2019-10-24
发表期刊	PHYSICAL REVIEW LETTERS
ISSN	0031-9007
EISSN	1079-7114
卷号	123 期号:17
发表状态	已发表
DOI	10.1103/PhysRevLett.123.173902
摘要	We report enhanced optical nonlinear effects at the surface of an ultrahigh-Q silica microcavity functionalized by a thin layer of organic molecules. The maximal conversion efficiency of third harmonic generation reaches similar to 1680%/W-2 and an absolute efficiency of 0.0144% at pump power of similar to 2.90 mW, which is approximately 4 orders of magnitude higher than that in a reported silica microcavity. Further analysis clarifies the elusive dependence of the third harmonic signal on the pump power in previous literature. Molecule-functionalized microcavities may find promising applications in high-efficiency broadband optical frequency conversion and offer potential in sensitive surface analysis.
收录类别	SCI ; SCIE ; EI
语种	英语
资助项目	China Postdoctoral Science Foundation[2018M640015]
WOS研究方向	Physics
WOS类目	Physics, Multidisciplinary
WOS记录号	WOS:000492373300004
出版者	AMER PHYSICAL SOC
EI主题词	Efficiency ; Microcavities ; Molecules ; Silica ; Surface analysis
WOS关键词	GENERATION ; RESONATOR ; EMISSION ; CHAOS
原始文献类型	Article
引用统计
文献类型	期刊论文
条目标识符	https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/80510
专题	物质科学与技术学院_PI研究组_沈晓钦组
通讯作者	Xiao, Yun-Feng
作者单位	1.Peking Univ, Sch Phys, State Key Lab Artificial Microstruct & Mesoscop P, Beijing 100871, Peoples R China 2.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China 3.Frontiers Sci Ctr Nanooptoelect, Beijing 100871, Peoples R China 4.Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China 5.Shanxi Univ, Collaborat Innovat Ctr Extreme Opt, Taiyuan 030006, Shanxi, Peoples R China 6.Beijing Acad Quantum Informat Sci, Beijing 100193, Peoples R China
推荐引用方式 GB/T 7714	Chen, Jin-hui,Shen, Xiaoqin,Tang, Shui-Jing,et al. Microcavity Nonlinear Optics with an Organically Functionalized Surface[J]. PHYSICAL REVIEW LETTERS,2019,123(17).
APA	Chen, Jin-hui,Shen, Xiaoqin,Tang, Shui-Jing,Cao, Qi-Tao,Gong, Qihuang,&Xiao, Yun-Feng.(2019).Microcavity Nonlinear Optics with an Organically Functionalized Surface.PHYSICAL REVIEW LETTERS,123(17).
MLA	Chen, Jin-hui,et al."Microcavity Nonlinear Optics with an Organically Functionalized Surface".PHYSICAL REVIEW LETTERS 123.17(2019).