Water-Degradable and Environmentally Responsive Mannich-Type Network
2025-01-21
状态已发表
摘要Polymer waste poses a significant challenge to humanity. In recent years, extensive efforts have been directed towards upcycling or degrading commercial polymers, as well as developing sustainable alternatives. However, limitations such as reliance on efficient waste collection systems and increased production costs persist. In this study, we introduce a strategy to address the challenges by developing mechanically robust polymer networks that degrade in water within 30 days. Utilizing three low-cost starting materials—guanidine hydrochloride, aldehyde, and diamine—our approach employs a Mannich-type reaction under mild condition. These polymer networks exhibit exceptional processability, enabling the fabrication of various forms, and demonstrate responsiveness to moisture, making them viable candidates for diverse applications. Our research paves the way for exploring an underexplored regime of polymer design, presenting a novel class of sustainable polymer networks.
关键词Mannich-type reaction polymer network degradable polymer moisture responsive guanidine
语种英语
DOI10.26434/chemrxiv-2025-fqt09
相关网址查看原文
出处chemRxiv
收录类别PPRN.PPRN
WOS记录号PPRN:120862268
WOS类目Chemistry, Multidisciplinary
资助项目Analytical Instrumentation Center at School of Physical Science and Technology, ShanghaiTech University[SPST-AIC10112914] ; National Natural Science Foundation of China[22401188] ; Science and Technology Commission of Shanghai Municipality[22YF1428200]
文献类型预印本
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/503594
专题物质科学与技术学院
物质科学与技术学院_本科生
生命科学与技术学院_博士生
物质科学与技术学院_博士生
物质科学与技术学院_PI研究组_严佳骏组
通讯作者Yan, Jiajun
作者单位
ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
推荐引用方式
GB/T 7714
Huang, Honglu,Liu, Hongjie,Cui, Feichen,et al. Water-Degradable and Environmentally Responsive Mannich-Type Network. 2025.
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