Hydrogenated metal oxide semiconductors for photoelectrochemical water splitting: Recent advances and future prospects

doi:10.1016/j.mser.2024.100918

KMS > 2060研究院 > 公共科研平台 > 分布式供能系统研究组

	Hydrogenated metal oxide semiconductors for photoelectrochemical water splitting: Recent advances and future prospects
	Xiaodan Wang1 ; Beibei Wang 2,3; Leonhard Mayrhofer 4; Xiangjian Meng 5; Hao Shen 2,3; Junhao Chu 2,3,5
	2025-04-01
发表期刊	MATERIALS SCIENCE & ENGINEERING R-REPORTS (IF:31.6[JCR-2023],34.3[5-Year])
ISSN	0927-796X
EISSN	1879-212X
卷号	163
DOI	10.1016/j.mser.2024.100918
摘要	Hydrogenated metal oxide semiconductors (HMOS) are witnessed tunable and superior structural, electrical, optical and catalytic properties, have emerged as a novel class of semiconductors in various applications, especially as photoanodes in photoelectrochemical (PEC) water splitting technology towards sustainable green hydrogen production, effectively overcoming the constraints associated with traditional metal oxides semiconductors which suffer limited visible light absorption and elevated electron-hole recombination rates. Herein, we offer a comprehensive overview of recent advances in fabrication, compositions and understanding of HMOS nanomaterials, as well as its crucial function in improving PEC activity, focusing on the potential hydrogenation techniques for practical applications and further surface and interface engineering strategies to boost PEC properties. We showcase a theoretical framework for understanding hydrogenation mechanisms and the impact on PEC activity. We also emphasize combining advanced and in-situ characterization techniques with theoretical simulations to unravel the mechanisms underlying the enhanced PEC activity to establish the structure-propertyfunction relationships from both macroscopic and microscopic perspectives. Finally, we discuss the remaining challenges in HMOS design and provide a perspective on further research directions of HMOS nanomaterials for PEC water splitting that realize PEC technology to contribute to produce green hydrogen efficiently.
关键词	Hydrogenated metal oxide semiconductors Photoelectrochemical water splitting Hydrogenation techniques Surface and interface engineering strategies Advanced and in-situ characterization tech- niques Density functional theory
URL	查看原文
收录类别	SCI ; EI
语种	英语
资助项目	COST (European Cooperation in Science and Technology)[IG18234]
WOS研究方向	Materials Science ; Physics
WOS类目	Materials Science, Multidisciplinary ; Physics, Applied
WOS记录号	WOS:001389565900001
出版者	ELSEVIER SCIENCE SA
EI入藏号	20245117529944
EI主题词	Hydrogenation
EI分类号	1501.1 Sustainable Development - 1501.2.1 Resource Conservation - 444 Water Resources - 701.1 Electricity: Basic Concepts and Phenomena - 802.2 Chemical Reactions - 804.1 Organic Compounds - 804.2 Inorganic Compounds - 901.3 Engineering Research
原始文献类型	Journal article (JA)
文献类型	期刊论文
条目标识符	https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/457908
专题	2060研究院_公共科研平台_分布式供能系统研究组
通讯作者	Xiaodan Wang; Hao Shen; Junhao Chu
作者单位	1.Institute of Carbon Neutrality, ShanghaiTech University, Huaxia Road No. 393, Shanghai 201210, China 2.Institute of Optoelectronics, Fudan University, Song Hu Road 2005, Shanghai 200438, China 3.Yiwu Research Institute, Fudan University, Zhongfu Square 5, Zhejiang 322000, China 4.Fraunhofer Institute for Mechanics of Materials IWM, Wöhlerstraße 11, Freiburg 79108, Germany 5.Fraunhofer Institute for Mechanics of Materials IWM, Wöhlerstraße 11, Freiburg 79108, Germany
第一作者单位	上海科技大学
通讯作者单位	上海科技大学
第一作者的第一单位	上海科技大学
推荐引用方式 GB/T 7714	Xiaodan Wang,Beibei Wang,Leonhard Mayrhofer,et al. Hydrogenated metal oxide semiconductors for photoelectrochemical water splitting: Recent advances and future prospects[J]. MATERIALS SCIENCE & ENGINEERING R-REPORTS,2025,163.
APA	Xiaodan Wang,Beibei Wang,Leonhard Mayrhofer,Xiangjian Meng,Hao Shen,&Junhao Chu.(2025).Hydrogenated metal oxide semiconductors for photoelectrochemical water splitting: Recent advances and future prospects.MATERIALS SCIENCE & ENGINEERING R-REPORTS,163.
MLA	Xiaodan Wang,et al."Hydrogenated metal oxide semiconductors for photoelectrochemical water splitting: Recent advances and future prospects".MATERIALS SCIENCE & ENGINEERING R-REPORTS 163(2025).