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Advanced X-ray spectroscopies: Unveiling chemical reaction mechanism in photo/electrocatalytic water splitting | |
2024-12-01 | |
发表期刊 | MATERIALS TODAY CHEMISTRY
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ISSN | 2468-5194 |
EISSN | 2468-5194 |
卷号 | 42 |
发表状态 | 已发表 |
DOI | 10.1016/j.mtchem.2024.102397 |
摘要 | The challenge of detecting intermediates in photo/electrocatalytic water splitting hinges critically on a profound understanding of processes across multiple spatial and temporal scales, encompassing electron excitation, electron transfer, interfacial reaction kinetics and so on. Advanced X-ray spectroscopies are powerful tools for analyzing complex processes at various scales. They offer non-destructive insights into electron dynamics, local structures, crystal lattices, and material distributions through absorption and imaging. This article provides an overview of the diverse applications of X-ray spectroscopies in the study of photo/electrocatalytic water splitting. It begins by introducing the fundamental principles of photo/electrocatalytic reactions for water splitting. Subsequently, it discusses the successful application of X-ray spectroscopic tools on the scales of energy resolution, temporal resolution, and spatial resolution in elucidating the mechanisms of chemical reactions in photo/ electrocatalytic water splitting. Finally, the review looks forward to the development of advanced X-ray spectroscopies and their potential applications in catalytic water splitting reactions. |
关键词 | X-ray spectroscopy In-situ / operando measurement Spectroscopic imaging Photo/electrocatalysis Water splitting |
URL | 查看原文 |
收录类别 | SCI ; EI |
语种 | 英语 |
资助项目 | National key research and development program["2019YFA0405601","2021YFA1500604"] ; National Natural Science Foundation of China[52130202] ; International Cooperation Project of 2022 Shanghai Action Plan for Science, Technology and Innovation[22560780300] |
WOS研究方向 | Chemistry ; Materials Science |
WOS类目 | Chemistry, Multidisciplinary ; Materials Science, Multidisciplinary |
WOS记录号 | WOS:001370631600001 |
出版者 | ELSEVIER SCI LTD |
EI入藏号 | 20244917457363 |
EI主题词 | Reaction intermediates |
EI分类号 | 1301.1.3.1 ; 741.3 Optical Devices and Systems ; 802.2 Chemical Reactions ; 804 Chemical Products Generally |
原始文献类型 | Journal article (JA) |
文献类型 | 期刊论文 |
条目标识符 | https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/452317 |
专题 | 大科学中心_公共科研平台_大科学装置建设部 物质科学与技术学院_硕士生 大科学中心_PI研究组_翁祖谦组 大科学中心 |
通讯作者 | Weng ZQ(翁祖谦) |
作者单位 | 1.上海科技大学物质学院 2.上海科技大学大科学中心 3.中国科学技术大学国家同步辐射实验室 |
第一作者单位 | 上海科技大学 |
通讯作者单位 | 上海科技大学; 大科学中心 |
第一作者的第一单位 | 上海科技大学 |
推荐引用方式 GB/T 7714 | Shen LF,Yu PF,Meng JW,et al. Advanced X-ray spectroscopies: Unveiling chemical reaction mechanism in photo/electrocatalytic water splitting[J]. MATERIALS TODAY CHEMISTRY,2024,42. |
APA | Shen LF,Yu PF,Meng JW,Liu XS,&Weng ZQ.(2024).Advanced X-ray spectroscopies: Unveiling chemical reaction mechanism in photo/electrocatalytic water splitting.MATERIALS TODAY CHEMISTRY,42. |
MLA | Shen LF,et al."Advanced X-ray spectroscopies: Unveiling chemical reaction mechanism in photo/electrocatalytic water splitting".MATERIALS TODAY CHEMISTRY 42(2024). |
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