Advanced X-ray spectroscopies: Unveiling chemical reaction mechanism in photo/electrocatalytic water splitting

doi:10.1016/j.mtchem.2024.102397

	Advanced X-ray spectroscopies: Unveiling chemical reaction mechanism in photo/electrocatalytic water splitting
	Shen LF(沈立夫)1 ; Yu PF(于鹏飞)2 ; Meng JW(孟建伟)2 ; Liu XS(刘啸嵩)3; Weng ZQ(翁祖谦)1,2
	2024-12-01
发表期刊	MATERIALS TODAY CHEMISTRY
ISSN	2468-5194
卷号	42
DOI	10.1016/j.mtchem.2024.102397
摘要	The challenge of detecting intermediates in photo/electrocatalytic water splitting hinges critically on a profound understanding of processes across multiple spatial and temporal scales, encompassing electron excitation, electron transfer, interfacial reaction kinetics and so on. Advanced X-ray spectroscopies are powerful tools for analyzing complex processes at various scales. They offer non-destructive insights into electron dynamics, local structures, crystal lattices, and material distributions through absorption and imaging. This article provides an overview of the diverse applications of X-ray spectroscopies in the study of photo/electrocatalytic water splitting. It begins by introducing the fundamental principles of photo/electrocatalytic reactions for water splitting. Subsequently, it discusses the successful application of X-ray spectroscopic tools on the scales of energy resolution, temporal resolution, and spatial resolution in elucidating the mechanisms of chemical reactions in photo/ electrocatalytic water splitting. Finally, the review looks forward to the development of advanced X-ray spectroscopies and their potential applications in catalytic water splitting reactions.
关键词	X-ray spectroscopy In-situ / operando measurement Spectroscopic imaging Photo/electrocatalysis Water splitting
URL	查看原文
收录类别	SCI
语种	英语
资助项目	National key research and development program["2019YFA0405601","2021YFA1500604"] ; National Natural Science Foundation of China[52130202] ; International Cooperation Project of 2022 Shanghai Action Plan for Science, Technology and Innovation[22560780300]
WOS研究方向	Chemistry ; Materials Science
WOS类目	Chemistry, Multidisciplinary ; Materials Science, Multidisciplinary
WOS记录号	WOS:001370631600001
出版者	ELSEVIER SCI LTD
文献类型	期刊论文
条目标识符	https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/452317
专题	大科学中心_公共科研平台_大科学装置建设部物质科学与技术学院_硕士生大科学中心_PI研究组_翁祖谦组大科学中心
通讯作者	Weng ZQ(翁祖谦)
作者单位	1.上海科技大学物质学院 2.上海科技大学大科学中心 3.中国科学技术大学国家同步辐射实验室
第一作者单位	上海科技大学
通讯作者单位	上海科技大学; 大科学中心
第一作者的第一单位	上海科技大学
推荐引用方式 GB/T 7714	Shen LF,Yu PF,Meng JW,et al. Advanced X-ray spectroscopies: Unveiling chemical reaction mechanism in photo/electrocatalytic water splitting[J]. MATERIALS TODAY CHEMISTRY,2024,42.
APA	Shen LF,Yu PF,Meng JW,Liu XS,&Weng ZQ.(2024).Advanced X-ray spectroscopies: Unveiling chemical reaction mechanism in photo/electrocatalytic water splitting.MATERIALS TODAY CHEMISTRY,42.
MLA	Shen LF,et al."Advanced X-ray spectroscopies: Unveiling chemical reaction mechanism in photo/electrocatalytic water splitting".MATERIALS TODAY CHEMISTRY 42(2024).