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Shortwave-Infrared Silver Chalcogenide Quantum Dots for Optoelectronic Devices
2024-10-01
发表期刊ACS NANO (IF:15.8[JCR-2023],16.2[5-Year])
ISSN1936-0851
EISSN1936-086X
卷号18期号:44页码:30123-30131
发表状态已发表
DOI10.1021/acsnano.4c11787
摘要

Silver chalcogenide (Ag2X, X = S, Se, Te) semiconductor quantum dots (QDs) have been extensively studied owing to their short-wave infrared (SWIR, 900-2500 nm) excitation and emission along with lower solubility product constant and environmentally benign nature. However, their unsatisfactory photoluminescence quantum yields (PLQYs) make it difficult to obtain optoelectronic devices with high performances. To tackle this challenge, researchers have made great efforts to develop valid strategies to improve the PLQYs of SWIR Ag2X QDs by suppressing their nonradiative recombination of excitons. In this Perspective, we summarize the significant approaches of heteroatom doping and surface passivation to enhance the PLQYs of SWIR Ag2X QDs, and we conclude their application in high-efficiency optoelectronic devices. Finally, we examine the future trends and promising opportunities of Ag2X QDs with regard to their optical properties and optoelectronics. We believe that this Perspective will serve as a valuable reference for future advancement in the synthesis and application of SWIR Ag2X QDs.

关键词short-wave infrared silver chalcogenide quantumdots photoluminescence quantum yields optoelectronics
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收录类别SCI ; EI
语种英语
资助项目National Natural Science Foundation of China[
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science
WOS类目Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号WOS:001340139300001
出版者AMER CHEMICAL SOC
EI入藏号20244517338372
EI主题词Photoluminescence
EI分类号202.7.1.2 ; 712.1.1 Single Element Semiconducting Materials ; 712.1.2 Compound Semiconducting Materials ; 714.2 Semiconductor Devices and Integrated Circuits ; 741.1 Light/Optics ; 741.3 Optical Devices and Systems ; 804 Chemical Products Generally ; 804.2 Inorganic Compounds
原始文献类型Journal article (JA)
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文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/445518
专题物质科学与技术学院_特聘教授组_王强斌组
通讯作者Wang, Qiangbin
作者单位
Chinese Acad Sci, Suzhou Inst Nanotech & Nanobion, Div Nanobiomedicine & I Lab, CAS Key Lab Nanobio Interface, Suzhou 215123, Peoples R China
推荐引用方式
GB/T 7714
Yang, Hongchao,Ma, Zhiwei,Wang, Qiangbin. Shortwave-Infrared Silver Chalcogenide Quantum Dots for Optoelectronic Devices[J]. ACS NANO,2024,18(44):30123-30131.
APA Yang, Hongchao,Ma, Zhiwei,&Wang, Qiangbin.(2024).Shortwave-Infrared Silver Chalcogenide Quantum Dots for Optoelectronic Devices.ACS NANO,18(44),30123-30131.
MLA Yang, Hongchao,et al."Shortwave-Infrared Silver Chalcogenide Quantum Dots for Optoelectronic Devices".ACS NANO 18.44(2024):30123-30131.
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