Dynamic Interpenetrating Polymer Network (IPN) Strategy for Multiresponsive Hierarchical Pattern of Reversible Wrinkle
2019-05
发表期刊ACS APPLIED MATERIALS & INTERFACES (IF:8.3[JCR-2023],8.7[5-Year])
ISSN1944-8244
卷号11期号:17页码:15977-15985
发表状态已发表
DOI10.1021/acsami.8b22216
摘要Dynamic micro-/nanowrinkle patterns with response to multienvironmental stimuli can offer a facile method for on-demand regulation of surface properties, thus allowing for generation of a smart surface. Here a practical yet robust strategy is described to fabricate redox, light and thermal responsive wrinkle by building dynamic double interpenetrating polymer network (IPN) as the top layer for a typical bilayer system. IPNs were constructed through the photochemical reaction of a mixture comprised of light-sensitive anthracene-containing polymer (PAN) and redox-sensitive disulfide-containing diacrylate monomer (DSDA). Thanks to the dynamic covalent reversible C-C bond in PAN and S-S bond in DSDA, the morphology of wrinkled surface not only can be reversibly and precisely (micrometer scale) tailored to all kinds of complicated hierarchical pattern permanently, but also can be controlled temporarily by irradiation of near-infrared light (NIR). A sine wave model is proposed to investigate the dynamics of real-time reversible wrinkle evolution. This general approach based on IPN allows independent multistimuli control over wettability and optical properties on the wrinkled surface, thus, presents a considerable alternative to implement a smart surface.
关键词interpenetrating polymer network surface pattern wrinkle multiresponsive dynamic chemistry
收录类别SCI ; SCIE ; EI
语种英语
资助项目Shanghai Municipal Government[17JC1400700] ; Shanghai Municipal Government[15SG13]
WOS研究方向Science & Technology - Other Topics ; Materials Science
WOS类目Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号WOS:000466988800090
出版者AMER CHEMICAL SOC
EI入藏号20191906894125
EI主题词Infrared devices ; Interpenetrating polymer networks ; Optical properties ; Photochemical reactions ; Polymers ; Sulfur compounds
EI分类号Light/Optics:741.1 ; Polymeric Materials:815.1 ; Materials Science:951
WOS关键词THIN-FILMS ; SURFACE ; MULTISTIMULI ; FABRICATION ; MODULATION ; METROLOGY ; FOLDS
原始文献类型Article
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文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/40881
专题物质科学与技术学院
通讯作者Jiang, Xuesong
作者单位
1.Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai Key Lab Elect Insulat & Thermal Ageing, State Key Lab Met Matrix Composite Mat, Shanghai 200240, Peoples R China
2.Shanghai Tech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
推荐引用方式
GB/T 7714
Zhou, Liangwei,Ma, Tianjiao,Li, Tiantian,et al. Dynamic Interpenetrating Polymer Network (IPN) Strategy for Multiresponsive Hierarchical Pattern of Reversible Wrinkle[J]. ACS APPLIED MATERIALS & INTERFACES,2019,11(17):15977-15985.
APA Zhou, Liangwei,Ma, Tianjiao,Li, Tiantian,Ma, Xiaodong,Yin, Jie,&Jiang, Xuesong.(2019).Dynamic Interpenetrating Polymer Network (IPN) Strategy for Multiresponsive Hierarchical Pattern of Reversible Wrinkle.ACS APPLIED MATERIALS & INTERFACES,11(17),15977-15985.
MLA Zhou, Liangwei,et al."Dynamic Interpenetrating Polymer Network (IPN) Strategy for Multiresponsive Hierarchical Pattern of Reversible Wrinkle".ACS APPLIED MATERIALS & INTERFACES 11.17(2019):15977-15985.
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