Electronic Correlation and Pseudogap-like Behavior of High-Temperature Superconductor La3Ni2O7
2024-07-10
发表期刊ARXIV (IF:3.5[JCR-2023],2.1[5-Year])
ISSN0256-307X
EISSN1741-3540
卷号41期号:8
发表状态已发表
DOIarXiv:2407.07501
摘要

High-temperature superconductivity (HTSC) remains one of the most challenging and fascinating mysteries in condensed matter physics. Recently, superconductivity with transition temperature exceeding liquid-nitrogen temperature is discovered in La3Ni2O7 at high pressure, which provides a new platform to explore the unconventional HTSC. In this work, using high-resolution angle-resolved photoemission spectroscopy and ab-initio calculation, we systematically investigate the electronic structures of La3Ni2O7 at ambient pressure. Our experiments are in nice agreement with ab-initio calculations after considering an orbital-dependent band renormalization effect. The strong electron correlation effect pushes a flat band of d_(z^2 ) orbital component below the Fermi level (EF), which is predicted to locate right at EF under high pressure. Moreover, the d_(x^2-y^2 ) band shows a pseudogap-like behavior with suppressed spectral weight and diminished quasiparticle peak near EF. Our findings provide important insights into the electronic structure of La3Ni2O7, which will shed light on the understanding of the unconventional superconductivity in nickelates.

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收录类别SCI
语种英语
资助项目National Key R&D Program of China["2022YFA1403100","2022YFA1403200"] ; National Natural Science Foundation of China["12275148","12004270","52272265"] ; Guangdong Basic and Applied Basic Research Foundation[2022B1515120020]
WOS研究方向Physics
WOS类目Physics, Condensed Matter
WOS记录号PPRN:90762952
出版者IOP Publishing Ltd
文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/408347
专题物质科学与技术学院
物质科学与技术学院_PI研究组_柳仲楷组
物质科学与技术学院_特聘教授组_陈宇林
物质科学与技术学院_PI研究组_齐彦鹏组
通讯作者Qi, Yanpeng
作者单位
1.Tsinghua Univ, Dept Phys, State Key Lab Low Dimens Quantum Phys, Beijing 100084, Peoples R China
2.Lanzhou Univ, Key Lab Magnetism & Magnet Mat, Minist Educ, Lanzhou 730000, Peoples R China
3.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
4.CAS, Shanghai Sci Res Ctr, Shanghai 201210, Peoples R China
5.ShanghaiTech Lab Topol Phys, Shanghai 200031, Peoples R China
6.Songshan Lake Mat Lab, Dongguan 523808, Guangdong, Peoples R China
7.Univ Oxford, Dept Phys, Clarendon Lab, Parks Rd, Oxford OX1 3PU, England
8.Frontier Sci Ctr Quantum Informat, Beijing 100084, Peoples R China
9.Collaborat Innovat Ctr Quantum Matter, Beijing 100084, Peoples R China
通讯作者单位物质科学与技术学院;  上海科技大学
推荐引用方式
GB/T 7714
Li, Yidian,Du, Xian,Cao, Yantao,et al. Electronic Correlation and Pseudogap-like Behavior of High-Temperature Superconductor La3Ni2O7[J]. ARXIV,2024,41(8).
APA Li, Yidian.,Du, Xian.,Cao, Yantao.,Pei, Cuiying.,Zhang, Mingxin.,...&Yang, Lexian.(2024).Electronic Correlation and Pseudogap-like Behavior of High-Temperature Superconductor La3Ni2O7.ARXIV,41(8).
MLA Li, Yidian,et al."Electronic Correlation and Pseudogap-like Behavior of High-Temperature Superconductor La3Ni2O7".ARXIV 41.8(2024).
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