WS2 ribbon arrays with defined chirality and coherent polarity
2024-06-07
发表期刊SCIENCE (IF:44.7[JCR-2023],50.3[5-Year])
ISSN0036-8075
EISSN1095-9203
卷号384期号:6700
发表状态已发表
DOI10.1126/science.adn9476
摘要

One-dimensional transition metal dichalcogenides exhibiting an enhanced bulk photovoltaic effect have the potential to exceed the Shockley-Queisser limit efficiency in solar energy harvest within p-n junction architectures. However, the collective output of these prototype devices remains a challenge. We report on the synthesis of single-crystalline WS2 ribbon arrays with defined chirality and coherent polarity through an atomic manufacturing strategy. The chirality of WS2 ribbon was defined by substrate couplings into tunable armchair, zigzag, and chiral species, and the polarity direction was determined by the ribbon-precursor interfacial energy along a coherent direction. A single armchair ribbon showed strong bulk photovoltaic effect and the further integration of similar to 1000 aligned ribbons with coherent polarity enabled upscaling of the photocurrent.

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收录类别SCI
语种英语
资助项目National Key R&D Program of China[2022YFA1403500] ; National Natural Science Foundation of China[
WOS研究方向Science & Technology - Other Topics
WOS类目Multidisciplinary Sciences
WOS记录号WOS:001253276700013
出版者AMER ASSOC ADVANCEMENT SCIENCE
引用统计
被引频次:13[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/398587
专题物质科学与技术学院
物质科学与技术学院_PI研究组_王竹君组
通讯作者Ding, Feng; Wei, Zhongming; Liu, Can; Liu, Kaihui
作者单位
1.Peking Univ, Frontiers Sci Ctr Nanooptoelect, State Key Lab Mesoscop Phys, Sch Phys,Acad Adv Interdisciplinary Studies, Beijing, Peoples R China
2.Renmin Univ China, Dept Phys, Minist Educ, Key Lab Quantum State Construct & Manipulat, Beijing, Peoples R China
3.Chinese Acad Sci, Inst Semicond, State Key Lab Superlatt & Microstruct, Beijing, Peoples R China
4.Peking Univ, Interdisciplinary Inst Light Element Quantum Mat, Beijing, Peoples R China
5.Peking Univ, Res Ctr Light Element Adv Mat, Beijing, Peoples R China
6.Kunming Univ Sci & Technol, Fac Met & Energy Engn, Kunming, Peoples R China
7.South China Normal Univ, Sch Phys & Telecommun Engn, Guangdong Prov Key Lab Quantum Engn & Quantum Mat, Guangzhou, Peoples R China
8.Chinese Acad Sci, Shenzhen Inst Adv Technol, Shenzhen, Peoples R China
9.Tsinghua Univ, Dept Engn Mech, Appl Mech Lab, Beijing, Peoples R China
10.Peking Univ, Int Ctr Quantum Mat, Collaborat Innovat Ctr Quantum Matter, Beijing, Peoples R China
11.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai, Peoples R China
12.Int Quantum Acad, Shenzhen, Peoples R China
13.Songshan Lake Mat Lab, Dongguan, Peoples R China
推荐引用方式
GB/T 7714
Xue, Guodong,Zhou, Ziqi,Guo, Quanlin,et al. WS2 ribbon arrays with defined chirality and coherent polarity[J]. SCIENCE,2024,384(6700).
APA Xue, Guodong.,Zhou, Ziqi.,Guo, Quanlin.,Zuo, Yonggang.,Wei, Wenya.,...&Liu, Kaihui.(2024).WS2 ribbon arrays with defined chirality and coherent polarity.SCIENCE,384(6700).
MLA Xue, Guodong,et al."WS2 ribbon arrays with defined chirality and coherent polarity".SCIENCE 384.6700(2024).
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