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Light-Boosting Highly Sensitive and Ultrafast Piezoelectric Sensor Based on Composite Membrane of Copper Phthalocyanine and Graphene Oxide
2024-06-01
发表期刊INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES (IF:4.9[JCR-2023],5.6[5-Year])
ISSN1661-6596
EISSN1422-0067
卷号25期号:12
发表状态已发表
DOI10.3390/ijms25126713
摘要Self-powered wearable pressure sensors based on flexible electronics have emerged as a new trend due to the increasing demand for intelligent and portable devices. Improvements in pressure-sensing performance, including in the output voltage, sensitivity and response time, can greatly expand their related applications; however, this remains challenging. Here, we report on a highly sensitive piezoelectric sensor with novel light-boosting pressure-sensing performance, based on a composite membrane of copper phthalocyanine (CuPC) and graphene oxide (GO) (CuPC@GO). Under light illumination, the CuPC@GO piezoelectric sensor demonstrates a remarkable increase in output voltage (381.17 mV, 50 kPa) and sensitivity (116.80 mV/kPa, <5 kPa), which are approximately twice and three times of that the sensor without light illumination, respectively. Furthermore, light exposure significantly improves the response speed of the sensor with a response time of 38.04 s and recovery time of 58.48 mu s, while maintaining excellent mechanical stability even after 2000 cycles. Density functional theory calculations reveal that increased electron transfer from graphene to CuPC can occur when the CuPC is in the excited state, which indicates that the light illumination promotes the electron excitation of CuPC, and thus brings about the high polarization of the sensor. Importantly, these sensors exhibit universal spatial non-contact adjustability, highlighting their versatility and applicability in various settings.
关键词piezoelectric sensor light illumination high sensitivity ultrafast response
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收录类别SCI
语种英语
资助项目National Natural Science Foundation of China["12004109","62103148"] ; Natural Science Foundation of Shanghai, China[23JC1401400]
WOS研究方向Biochemistry & Molecular Biology ; Chemistry
WOS类目Biochemistry & Molecular Biology ; Chemistry, Multidisciplinary
WOS记录号WOS:001257141500001
出版者MDPI
文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/398580
专题大科学中心_PI研究组_刘志组
通讯作者Gu, Zhen; Fang, Haiping
作者单位
1.East China Univ Sci & Technol, Sch Phys, Shanghai 200237, Peoples R China
2.East China Univ Sci & Technol, Sch Mat Sci & Engn, Shanghai 200237, Peoples R China
3.ShanghaiTech Univ, Ctr Transformat Sci, Shanghai 200237, Peoples R China
4.East China Univ Sci & Technol, Key Lab Smart Mfg Energy Chem Proc, Minist Educ, Shanghai 200237, Peoples R China
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GB/T 7714
Wang, Jihong,Fang, Zhening,Liu, Wenhao,et al. Light-Boosting Highly Sensitive and Ultrafast Piezoelectric Sensor Based on Composite Membrane of Copper Phthalocyanine and Graphene Oxide[J]. INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES,2024,25(12).
APA Wang, Jihong.,Fang, Zhening.,Liu, Wenhao.,Zhu, Liuyuan.,Pan, Qiubo.,...&Fang, Haiping.(2024).Light-Boosting Highly Sensitive and Ultrafast Piezoelectric Sensor Based on Composite Membrane of Copper Phthalocyanine and Graphene Oxide.INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES,25(12).
MLA Wang, Jihong,et al."Light-Boosting Highly Sensitive and Ultrafast Piezoelectric Sensor Based on Composite Membrane of Copper Phthalocyanine and Graphene Oxide".INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES 25.12(2024).
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