Optical signatures of type-II Weyl fermions in the noncentrosymmetric semimetals RAlSi (R=La, Ce, Pr, Nd, Sm)
2024-05-15
发表期刊PHYSICAL REVIEW B (IF:3.2[JCR-2023],3.3[5-Year])
ISSN2469-9950
EISSN2469-9969
卷号109期号:19
发表状态已发表
DOI10.1103/PhysRevB.109.195130
摘要Weyl semimetals with magnetic ordering provide a promising platform for the investigation of rare topological effects such as the anomalous Hall effect, resulting from the interplay of nontrivial bands with various spin configurations. The materials RAlSi, where R represents a rare-earth element, are prominent representatives of Weyl semimetals, where the Weyl states are induced by space inversion symmetry breaking, and in addition, for several rare-earth elements R, enhanced by time-reversal symmetry breaking through the formation of a magnetic order at low temperature. We report optical signatures of Weyl fermions in the magnetic compounds CeAlSi, PrAlSi, NdAlSi, and SmAlSi as well as the nonmagnetic family member LaAlSi by broad-frequency infrared spectroscopy at room temperature, i.e., in the paramagnetic phase. A similar profile of the optical conductivity spectrum and a metallic character are observed for all compounds, with LaAlSi showing the strongest free charge-carrier contribution. Furthermore, the linear-in-frequency behavior of the optical conductivity of all investigated compounds indicates the presence of Weyl nodes in close proximity to the Fermi energy, resulting from inversion symmetry breaking in noncentrosymmetric structures. According to the characteristics of these linear slopes, the RAlSi compounds are expected to host mainly type-II Weyl states with overtilted Weyl cones. The results are compared to the optical response of the closely related RAlGe materials, which are considered as potential hybridization-driven Weyl-Kondo systems. © 2024 American Physical Society.
关键词Heterojunctions Infrared spectroscopy Lanthanum compounds Rare earth elements Silicon compounds Temperature Anomalous hall effects Inversion symmetry Lows-temperatures Magnetic orders Optical signatures Spin configurations Symmetry breakings Time reversal symmetries Topological effects Type II
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收录类别EI ; SCI
语种英语
资助项目Deutsche Forschungsgemeinschaft (DFG, German Research Foundation)[TRR 360-492547816] ; National Natural Science Foundation of China["52272265","U1932217","11974246","12004252"] ; National Key R & D Program of China[2018YFA0704300]
WOS研究方向Materials Science ; Physics
WOS类目Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS记录号WOS:001237461200001
出版者American Physical Society
EI入藏号20242016088800
EI主题词Rare earths
EI分类号547.2 Rare Earth Metals ; 641.1 Thermodynamics ; 714.2 Semiconductor Devices and Integrated Circuits ; 804.2 Inorganic Compounds
原始文献类型Journal article (JA)
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文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/375717
专题物质科学与技术学院
物质科学与技术学院_PI研究组_齐彦鹏组
物质科学与技术学院_博士生
作者单位
1.Experimental Physics II, Institute of Physics, University of Augsburg, Augsburg; 86159, Germany;
2.School of Physical Science and Technology, ShanghaiTech University, Shanghai; 201210, China;
3.ShanghaiTech Laboratory for Topological Physics, ShanghaiTech University, Shanghai; 201210, China;
4.Shanghai Key Laboratory of High-resolution Electron Microscopy, Shanghai Tech Laboratory for Topological Physics, Shanghai Tech University, Shanghai; 201210, China
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Kunze, J.,Köpf, M.,Cao, Weizheng,et al. Optical signatures of type-II Weyl fermions in the noncentrosymmetric semimetals RAlSi (R=La, Ce, Pr, Nd, Sm)[J]. PHYSICAL REVIEW B,2024,109(19).
APA Kunze, J.,Köpf, M.,Cao, Weizheng,Qi, Yanpeng,&Kuntscher, C.A..(2024).Optical signatures of type-II Weyl fermions in the noncentrosymmetric semimetals RAlSi (R=La, Ce, Pr, Nd, Sm).PHYSICAL REVIEW B,109(19).
MLA Kunze, J.,et al."Optical signatures of type-II Weyl fermions in the noncentrosymmetric semimetals RAlSi (R=La, Ce, Pr, Nd, Sm)".PHYSICAL REVIEW B 109.19(2024).
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