Attosecond-resolved non-dipole photoionization dynamics
2024
发表期刊NATURE PHOTONICS (IF:32.3[JCR-2023],35.8[5-Year])
ISSN1749-4885
EISSN1749-4893
卷号18期号:4页码:311-317
发表状态已发表
DOI10.1038/s41566-023-01349-z
摘要

Light–matter interactions are usually described within the electric-dipole approximation, where the magnetic-field component and the spatial variation of the light electric field over the relevant electronic length scales are both ignored. Non-dipole effects in photoionization were revealed to be tiny from the infrared to the soft X-ray domains, and all non-dipole observations reported so far were limited to single-pulse, single-colour measurements. Here we advance attosecond time-resolved spectroscopy into the non-dipole interaction regime. Using a self-referenced attosecond photoelectron interferometry on helium atoms, we resolve the electron subcycle motion along the light propagation direction in the 15 pm range driven by the magnetic component of a near-infrared laser field. Furthermore, we measure a time delay of 15 ± 10 as between the electric-dipole and electric-quadrupole transitions by resolving the asymmetry of the photoelectron forward–backward yields with attosecond resolution. These fundamental findings are supported by ab initio calculations based on the non-dipole time-dependent Schrödinger equation. © 2024, The Author(s), under exclusive licence to Springer Nature Limited.

关键词Atom lasers Electric fields Infrared devices Infrared lasers Laser spectroscopy Photoionization Photons Attoseconds Electric-dipole approximation Length scale Light-matter interactions Magnetic field components Non-dipole Nondipole effect Photoionization dynamics Soft X-ray Spatial variations
收录类别EI
语种英语
出版者Nature Research
EI入藏号20240215373540
EI主题词Photoelectrons
EI分类号701.1 Electricity: Basic Concepts and Phenomena ; 711 Electromagnetic Waves ; 741.3 Optical Devices and Systems ; 744.1 Lasers, General ; 744.9 Laser Applications ; 802.2 Chemical Reactions ; 931.3 Atomic and Molecular Physics ; 941.4 Optical Variables Measurements
原始文献类型Article in Press
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文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/348637
专题物质科学与技术学院
大科学中心
通讯作者Han, Meng; Zhou, Yueming; Lu, Peixiang
作者单位
1.Wuhan National Laboratory for Optoelectronics and School of Physics, Huazhong University of Science and Technology, Wuhan, China
2.Laboratorium für Physikalische Chemie, ETH Zürich, Zürich, Switzerland
3.J. R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan; KS, United States
4.Institute of Quantum Precision Measurement, College of Physics and Optoelectronic Engineering, Shenzhen University, Shenzhen, China
5.Department of Chemistry, Tohoku University, Sendai, Japan
6.School of Physical Science and Technology, ShanghaiTech University, Shanghai, China
7.Optics Valley Laboratory, Hubei, China
推荐引用方式
GB/T 7714
Liang, Jintai,Han, Meng,Liao, Yijie,et al. Attosecond-resolved non-dipole photoionization dynamics[J]. NATURE PHOTONICS,2024,18(4):311-317.
APA Liang, Jintai.,Han, Meng.,Liao, Yijie.,Ji, Jia-bao.,Leung, Chung Sum.,...&Wörner, Hans Jakob.(2024).Attosecond-resolved non-dipole photoionization dynamics.NATURE PHOTONICS,18(4),311-317.
MLA Liang, Jintai,et al."Attosecond-resolved non-dipole photoionization dynamics".NATURE PHOTONICS 18.4(2024):311-317.
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