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Attosecond-resolved non-dipole photoionization dynamics | |
2024 | |
发表期刊 | NATURE PHOTONICS (IF:32.3[JCR-2023],35.8[5-Year]) |
ISSN | 1749-4885 |
EISSN | 1749-4893 |
卷号 | 18期号:4页码:311-317 |
发表状态 | 已发表 |
DOI | 10.1038/s41566-023-01349-z |
摘要 | Light–matter interactions are usually described within the electric-dipole approximation, where the magnetic-field component and the spatial variation of the light electric field over the relevant electronic length scales are both ignored. Non-dipole effects in photoionization were revealed to be tiny from the infrared to the soft X-ray domains, and all non-dipole observations reported so far were limited to single-pulse, single-colour measurements. Here we advance attosecond time-resolved spectroscopy into the non-dipole interaction regime. Using a self-referenced attosecond photoelectron interferometry on helium atoms, we resolve the electron subcycle motion along the light propagation direction in the 15 pm range driven by the magnetic component of a near-infrared laser field. Furthermore, we measure a time delay of 15 ± 10 as between the electric-dipole and electric-quadrupole transitions by resolving the asymmetry of the photoelectron forward–backward yields with attosecond resolution. These fundamental findings are supported by ab initio calculations based on the non-dipole time-dependent Schrödinger equation. © 2024, The Author(s), under exclusive licence to Springer Nature Limited. |
关键词 | Atom lasers Electric fields Infrared devices Infrared lasers Laser spectroscopy Photoionization Photons Attoseconds Electric-dipole approximation Length scale Light-matter interactions Magnetic field components Non-dipole Nondipole effect Photoionization dynamics Soft X-ray Spatial variations |
收录类别 | EI |
语种 | 英语 |
出版者 | Nature Research |
EI入藏号 | 20240215373540 |
EI主题词 | Photoelectrons |
EI分类号 | 701.1 Electricity: Basic Concepts and Phenomena ; 711 Electromagnetic Waves ; 741.3 Optical Devices and Systems ; 744.1 Lasers, General ; 744.9 Laser Applications ; 802.2 Chemical Reactions ; 931.3 Atomic and Molecular Physics ; 941.4 Optical Variables Measurements |
原始文献类型 | Article in Press |
引用统计 | 正在获取...
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文献类型 | 期刊论文 |
条目标识符 | https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/348637 |
专题 | 物质科学与技术学院 大科学中心 |
通讯作者 | Han, Meng; Zhou, Yueming; Lu, Peixiang |
作者单位 | 1.Wuhan National Laboratory for Optoelectronics and School of Physics, Huazhong University of Science and Technology, Wuhan, China 2.Laboratorium für Physikalische Chemie, ETH Zürich, Zürich, Switzerland 3.J. R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan; KS, United States 4.Institute of Quantum Precision Measurement, College of Physics and Optoelectronic Engineering, Shenzhen University, Shenzhen, China 5.Department of Chemistry, Tohoku University, Sendai, Japan 6.School of Physical Science and Technology, ShanghaiTech University, Shanghai, China 7.Optics Valley Laboratory, Hubei, China |
推荐引用方式 GB/T 7714 | Liang, Jintai,Han, Meng,Liao, Yijie,et al. Attosecond-resolved non-dipole photoionization dynamics[J]. NATURE PHOTONICS,2024,18(4):311-317. |
APA | Liang, Jintai.,Han, Meng.,Liao, Yijie.,Ji, Jia-bao.,Leung, Chung Sum.,...&Wörner, Hans Jakob.(2024).Attosecond-resolved non-dipole photoionization dynamics.NATURE PHOTONICS,18(4),311-317. |
MLA | Liang, Jintai,et al."Attosecond-resolved non-dipole photoionization dynamics".NATURE PHOTONICS 18.4(2024):311-317. |
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