Three dimensional porous Cu-Zn/Al foam monolithic catalyst for CO2 hydrogenation to methanol in microreactor

doi:10.1016/j.jcou.2017.05.023

	Three dimensional porous Cu-Zn/Al foam monolithic catalyst for CO2 hydrogenation to methanol in microreactor
	Liang, Zhuangdian1,2,3 ; Gao, Peng 1; Tang, Zhiyong 1; Lv, Min 1; Sun, Yuhan1,3
	2017-10
发表期刊	JOURNAL OF CO2 UTILIZATION (IF:7.2[JCR-2023],7.4[5-Year])
ISSN	2212-9820
卷号	21 页码:191-199
发表状态	已发表
DOI	10.1016/j.jcou.2017.05.023
摘要	CO2 hydrogenation turns to be an attractive pathway of C1 conversion. For CO2 hydrogenation to methanol, a novel method was investigated for the preparation of layer structured Cu-Zn/Al foam monolithic catalyst integrated with microreactor. Such a monolithic catalyst could be loaded in a flange-type microreactor in the form of packed bed to intensify the process. As a result, a high copper time yield of methanol, 7.81 g g(Cu)(-1) h(-1), was obtained at 250 degrees C, 3 MPa and 20000 mL g(cat)(-1) h(-1) due to the heat/mass-transfer properties with microreactor. Besides, the monolithic catalyst showed a good ability of adhesion.
关键词	Carbon dioxide hydrogenation Copper-based catalyst Methanol synthesis Monolithic catalyst Microreactor
收录类别	SCI ; EI
语种	英语
资助项目	Shanghai Municipal Science and Technology Commission, China[16DZ1206900]
WOS研究方向	Chemistry ; Engineering
WOS类目	Chemistry, Multidisciplinary ; Engineering, Chemical
WOS记录号	WOS:000411443200022
出版者	ELSEVIER SCI LTD
EI入藏号	20173003991921
EI主题词	Carbon ; Carbon dioxide ; Chemical reactors ; Copper ; Hydrogenation ; Methanol ; Packed beds ; Synthesis gas manufacture
EI分类号	Copper:544.1 ; Chemical Plants and Equipment:802.1 ; Chemical Reactions:802.2 ; Chemical Products Generally:804
WOS关键词	HYDROTALCITE-LIKE PRECURSORS ; FISCHER-TROPSCH SYNTHESIS ; CARBON-DIOXIDE ; CU/ZN/AL/ZR CATALYSTS ; PERFORMANCE ; CONVERSION ; CU/ZNO/AL2O3 ; GLYCEROL ; ALUMINA ; OXIDES
原始文献类型	Article
引用统计	正在获取...
文献类型	期刊论文
条目标识符	https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/2817
专题	物质科学与技术学院物质科学与技术学院_特聘教授组_孙予罕组物质科学与技术学院_硕士生
通讯作者	Lv, Min; Sun, Yuhan
作者单位	1.Chinese Acad Sci, Shanghai Adv Res Inst, CAS Key Lab Low Carbon Convers Sci & Engn, 99 Haike Rd,Zhangjiang Hitech Pk, Shanghai 201210, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
第一作者单位	物质科学与技术学院
通讯作者单位	物质科学与技术学院
推荐引用方式 GB/T 7714	Liang, Zhuangdian,Gao, Peng,Tang, Zhiyong,et al. Three dimensional porous Cu-Zn/Al foam monolithic catalyst for CO2 hydrogenation to methanol in microreactor[J]. JOURNAL OF CO2 UTILIZATION,2017,21:191-199.
APA	Liang, Zhuangdian,Gao, Peng,Tang, Zhiyong,Lv, Min,&Sun, Yuhan.(2017).Three dimensional porous Cu-Zn/Al foam monolithic catalyst for CO2 hydrogenation to methanol in microreactor.JOURNAL OF CO2 UTILIZATION,21,191-199.
MLA	Liang, Zhuangdian,et al."Three dimensional porous Cu-Zn/Al foam monolithic catalyst for CO2 hydrogenation to methanol in microreactor".JOURNAL OF CO2 UTILIZATION 21(2017):191-199.