CO2 capture from humid flue gases and humid atmosphere using a microporous coppersilicate

doi:10.1126/science.aab1680

KMS > 物质科学与技术学院 > PI研究组 > Osamu Terasaki组

	CO2 capture from humid flue gases and humid atmosphere using a microporous coppersilicate
	Datta, Shuvo Jit 1; Khumnoon, Chutharat 1; Lee, Zhen Hao 1; Moon, Won Kyung 1; Docao, Son 1; Nguyen, Thanh Huu 1; Hwang, In Chul 1; Moon, Dohyun 2; Oleynikov, Peter 3; Terasaki, Osamu3,4,5 ; Yoon, Kyung Byung 1
	2015-10-16
发表期刊	SCIENCE (IF:44.7[JCR-2023],50.3[5-Year])
ISSN	0036-8075
卷号	350 期号:6258 页码:302-+
发表状态	已发表
DOI	10.1126/science.aab1680
摘要	Capturing CO2 from humid flue gases and atmosphere with porous materials remains costly because prior dehydration of the gases is required. A large number of microporous materials with physical adsorption capacity have been developed as CO2-capturing materials. However, most of them suffer from CO2 sorption capacity reduction or structure decomposition that is caused by co-adsorbed H2O when exposed to humid flue gases and atmosphere. We report a highly stable microporous coppersilicate. It has H2O-specific and CO2-specific adsorption sites but does not have H2O/CO2-sharing sites. Therefore, it readily adsorbs both H2O and CO2 from the humid flue gases and atmosphere, but the adsorbing H2O does not interfere with the adsorption of CO2. It is also highly stable after adsorption of H2O and CO2 because it was synthesized hydrothermally.
收录类别	SCI
语种	英语
资助项目	Ministry of Science, ICT and Future Planning through the National Research Foundation of Korea[2009-0093886]
WOS研究方向	Science & Technology - Other Topics
WOS类目	Multidisciplinary Sciences
WOS记录号	WOS:000362838700036
出版者	AMER ASSOC ADVANCEMENT SCIENCE
WOS关键词	METAL-ORGANIC FRAMEWORK ; CARBON-DIOXIDE CAPTURE ; POROUS MATERIALS ; ADSORPTION ; ADSORBENTS ; SEPARATION
原始文献类型	Article
引用统计	正在获取...
文献类型	期刊论文
条目标识符	https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/2471
专题	物质科学与技术学院_PI研究组_Osamu Terasaki组
通讯作者	Yoon, Kyung Byung
作者单位	1.Sogang Univ, Dept Chem, Korea Ctr Artificial Photosynthesis, Seoul 121742, South Korea 2.Pohang Univ Sci & Technol, Pohang Accelerator Lab, Pohang 790784, South Korea 3.Stockholm Univ, Dept Mat & Environm Chem, SE-10691 Stockholm, Sweden 4.Korea Adv Inst Sci & Technol, Grad Sch EEWS, Taejon 305701, South Korea 5.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
推荐引用方式 GB/T 7714	Datta, Shuvo Jit,Khumnoon, Chutharat,Lee, Zhen Hao,et al. CO2 capture from humid flue gases and humid atmosphere using a microporous coppersilicate[J]. SCIENCE,2015,350(6258):302-+.
APA	Datta, Shuvo Jit.,Khumnoon, Chutharat.,Lee, Zhen Hao.,Moon, Won Kyung.,Docao, Son.,...&Yoon, Kyung Byung.(2015).CO2 capture from humid flue gases and humid atmosphere using a microporous coppersilicate.SCIENCE,350(6258),302-+.
MLA	Datta, Shuvo Jit,et al."CO2 capture from humid flue gases and humid atmosphere using a microporous coppersilicate".SCIENCE 350.6258(2015):302-+.