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A Simple Framework for Quantifying Electrochemical CO2 Fixation
2018-04-18
发表期刊JOULE (IF:38.6[JCR-2023],44.8[5-Year])
ISSN2542-4351
卷号2期号:4页码:594-606
发表状态已发表
DOI10.1016/j.joule.2018.02.003
摘要Substantial abatements of CO2 emissions from fossil fuel combustions are critical to shifting the current trend of fast global warming. In this Perspective, chemical fixation of CO2 (CFC) is evaluated as a progressive abating strategy by a proposed "golden triangle'' principle. We derive several simple equations to describe partially the relationships between energy and CO2 arising from fossil fuel combustions in the power sector upon energy/mass-balance analyses of related electrochemical reductions of CO2 (ERCs) as a route to CFC. Mitigation coefficients are obtained as figures of merit to quantify the intrinsic abatement capabilities of various reduction products, identifying privileged ERCs that may allow fossil fuel power, the current and expected dominant source of electricity at least before 2040, to drive the ERCs for emission abatements. The challenges for large-scale deployments of the ERCs as a substantial emission-abating strategy are discussed upon sensitivity analysis of mitigation efficiency for selected privileged ERCs.
收录类别EI ; SCIE ; ESCI ; SCI
语种英语
WOS研究方向Energy & Fuels
WOS类目Energy & Fuels
WOS记录号WOS:000435091900009
出版者CELL PRESS
EI入藏号20181404981841
EI主题词Bioassay ; Budget control ; Chemical analysis ; Costs ; Electrolytic reduction ; Fossil fuels ; Fuel storage ; Global warming ; Greenhouse gases ; Industrial emissions ; Sensitivity analysis
WOS关键词CARBON-DIOXIDE ; LOW-COST ; REDUCTION ; METAL
原始文献类型Review
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文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/20210
专题物质科学与技术学院_PI研究组_林柏霖组
物质科学与技术学院
物质科学与技术学院_本科生
通讯作者Lin, Bo-Lin
作者单位
School of Physical Science and Technology, ShanghaiTech University, 393 Middle Huaxia Road, Shanghai; 201210, China
第一作者单位物质科学与技术学院
通讯作者单位物质科学与技术学院
第一作者的第一单位物质科学与技术学院
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GB/T 7714
Chen, Anqi,Lin, Bo-Lin. A Simple Framework for Quantifying Electrochemical CO2 Fixation[J]. JOULE,2018,2(4):594-606.
APA Chen, Anqi,&Lin, Bo-Lin.(2018).A Simple Framework for Quantifying Electrochemical CO2 Fixation.JOULE,2(4),594-606.
MLA Chen, Anqi,et al."A Simple Framework for Quantifying Electrochemical CO2 Fixation".JOULE 2.4(2018):594-606.
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