Signatures of spin-orbit coupling and charge localization in CrIr2Sn10: a scanning tunneling microscope study
2022-06-02
发表期刊THE JOURNAL OF PHYSICAL CHEMISTRY C (IF:3.3[JCR-2023],3.5[5-Year])
ISSN1932-7447
EISSN1932-7455
卷号126期号:21页码:9117-9122
发表状态正式接收
DOI10.1021/acs.jpcc.1c10654
摘要

Magnetic topological insulators and semimetals have become an import branch in the study of topological materials. Topological materials with intrinsic magnetism are superior for better quality and performances. Here we report a scanning tunneling microscopic study of CrIr2Sn10, a newly synthesized material as a candidate for magnetic topological semimetal. Sn and Cr surface terminations are identified with distinctive spectroscopic characters. Charge localization is signified by the density of states peak near -200 meV that is consistent with the flat band dispersion in density functional theory calculations. The electron correlations are further evidenced by the particle-hole asymmetry in the background of differential conductance spectrum. The inserting of Cr layers not only introduces ferromagnetism in the material, but also breaks the local inversion symmetry of Sn-Ir-Sn unit structure compared with IrSn4. The spin-orbit coupling thus induced/enhanced is essential to the band topologies. Our findings suggest that CrIr2Sn10 could be an ideal platform for exploring the symmetry-protected topological phases as well as their interplay with electron correlation and magnetism.

关键词Chromium Chromium alloys Iridium alloys Iridium compounds Ternary alloys Tin alloys Topology Band dispersions Charge localization Densities of state Flat band Microscopic study Performance Spin-orbit couplings Surface termination Synthesized materials Topological materials
收录类别SCI ; SCIE ; EI
语种英语
出版者American Chemical Society
EI入藏号20222412217317
EI主题词Density functional theory
EI分类号543.1 Chromium and Alloys ; 546.2 Tin and Alloys ; 547.1 Precious Metals ; 921.4 Combinatorial Mathematics, Includes Graph Theory, Set Theory ; 922.1 Probability Theory ; 931.3 Atomic and Molecular Physics ; 931.4 Quantum Theory ; Quantum Mechanics
原始文献类型Journal article (JA)
文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/178465
专题物质科学与技术学院_硕士生
物质科学与技术学院_特聘教授组_乔山组
共同第一作者Fang Yuqiang; Li Ang
通讯作者Li Ang
作者单位
1.School of Physical Science and Technology, ShanghaiTech University
2.State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences
3.State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences
4.Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences
第一作者单位物质科学与技术学院
第一作者的第一单位物质科学与技术学院
推荐引用方式
GB/T 7714
Li Kaiyi,Fang Yuqiang,Zha Heming,et al. Signatures of spin-orbit coupling and charge localization in CrIr2Sn10: a scanning tunneling microscope study[J]. THE JOURNAL OF PHYSICAL CHEMISTRY C,2022,126(21):9117-9122.
APA Li Kaiyi.,Fang Yuqiang.,Zha Heming.,Liu Jianzhong.,Ma Ni.,...&Li Ang.(2022).Signatures of spin-orbit coupling and charge localization in CrIr2Sn10: a scanning tunneling microscope study.THE JOURNAL OF PHYSICAL CHEMISTRY C,126(21),9117-9122.
MLA Li Kaiyi,et al."Signatures of spin-orbit coupling and charge localization in CrIr2Sn10: a scanning tunneling microscope study".THE JOURNAL OF PHYSICAL CHEMISTRY C 126.21(2022):9117-9122.
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