Sizes of pure and doped helium droplets from single shot x-ray imaging

doi:10.1063/5.0080342

	Sizes of pure and doped helium droplets from single shot x-ray imaging
	Tanyag, Rico Mayro P.1,19; Bacellar, Camila 2,3,17; Pang, Weiwu 4; Bernando, Charles 5,20; Gomez, Luis F.1; Jones, Curtis F.1,21; Ferguson, Ken R.6; Kwok, Justin 7,22; Anielski, Denis 8; Belkacem, Ali 2; Boll, Rebecca 8,23; Bozek, John 6; Carron, Sebastian 6; Chen, Gang9,24 ; Delmas, Tjark 10; Englert, Lars 11,25; Epp, Sascha W.8,26; Erk, Benjamin 8,27; Foucar, Lutz 12; Hartmann, Robert 13; Hexemer, Alexander 9; Huth, Martin 13,28; Leone, Stephen R.2,3; Ma, Jonathan H.2; Marchesini, Stefano 9,14; Neumark, Daniel M.2,3; Poon, Billy K.15,29; Prell, James 2,3; Rolles, Daniel 8,16; Rudek, Benedikt 8,30; Rudenko, Artem 8,16; Seifrid, Martin ; Swiggers, Michele 6; Ullrich, Joachim 8,31; Weise, Fabian 2; Zwart, Petrus 15,32; Bostedt, Christoph 6,17,18; Gessner, Oliver 2; Vilesov, Andrey F.1,5
	2022-01-28
发表期刊	JOURNAL OF CHEMICAL PHYSICS (IF:3.1[JCR-2023],3.6[5-Year])
ISSN	0021-9606
EISSN	1089-7690
卷号	156 期号:4
发表状态	已发表
DOI	10.1063/5.0080342
摘要	Advancements in x-ray free-electron lasers on producing ultrashort, ultrabright, and coherent x-ray pulses enable single-shot imaging of fragile nanostructures, such as superfluid helium droplets. This imaging technique gives unique access to the sizes and shapes of individual droplets. In the past, such droplet characteristics have only been indirectly inferred by ensemble averaging techniques. Here, we report on the size distributions of both pure and doped droplets collected from single-shot x-ray imaging and produced from the free-jet expansion of helium through a 5 μm diameter nozzle at 20 bars and nozzle temperatures ranging from 4.2 to 9 K. This work extends the measurement of large helium nanodroplets containing 109-1011 atoms, which are shown to follow an exponential size distribution. Additionally, we demonstrate that the size distributions of the doped droplets follow those of the pure droplets at the same stagnation condition but with smaller average sizes. © 2022 Author(s).
关键词	Drops Electrons Free electron lasers Spray nozzles Superfluid helium Coherent X-rays Helium droplets Single-shot Single-shot imaging Size and shape Size-distribution Superfluid helium droplets X ray pulse X-ray free electron lasers Xray imaging
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收录类别	SCI ; SCIE ; EI
语种	英语
资助项目	NSF[
WOS研究方向	Chemistry ; Physics
WOS类目	Chemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS记录号	WOS:000755084400006
出版者	American Institute of Physics Inc.
EI入藏号	20220611607062
EI主题词	Size distribution
EI分类号	631.1 Fluid Flow, General ; 744.5 Free Electron Lasers ; 804 Chemical Products Generally ; 922.2 Mathematical Statistics
原始文献类型	Journal article (JA)
引用统计	正在获取...
文献类型	期刊论文
条目标识符	https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/154112
专题	物质科学与技术学院_PI研究组_陈刚组
通讯作者	Tanyag, Rico Mayro P.; Vilesov, Andrey F.
作者单位	1.Univ Southern Calif, Dept Chem, Los Angeles, CA 90089 USA 2.Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA 3.Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA 4.Univ Southern Calif, Dept Comp Sci, Los Angeles, CA 90089 USA 5.Univ Southern Calif, Dept Phys & Astron, Los Angeles, CA 90089 USA 6.SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA 7.Univ Southern Calif, Dept Chem Engn & Mat Sci, Los Angeles, CA 90089 USA 8.Max Planck Inst Kernphys, Saupfercheckweg 1, D-69117 Heidelberg, Germany 9.Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA 10.Deutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci CFEL, Notkestr 85, D-22607 Hamburg, Germany 11.Max Planck Inst Extraterr Phys, Giessenbachstr, D-85741 Garching, Germany 12.Max Planck Inst Med Res, Jahnstr 29, D-69120 Heidelberg, Germany 13.PNSensor GmbH, Otto Hahn Ring 6, D-81739 Munich, Germany 14.Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA 15.Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA 16.Kansas State Univ, Dept Phys, JR MacDonald Lab, Manhattan, KS 66506 USA 17.Paul Scherrer Inst, CH-5232 Villigen, Switzerland 18.Ecole Polytech Fed Lausanne EPFL, Inst Chem Sci & Engn, LUXS Lab Ultrafast Xray Sci, CH-1015 Lausanne, Switzerland 19.Aarhus Univ, Dept Chem, DK-8000 Aarhus C, Denmark 20.BINUS Univ, Sch Informat Syst, Jl KH Syahdan 9, Jakarta 11480, Indonesia 21.SUNY Adirondack, Queensbury, NY 12804 USA 22.Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA 23.European XFEL, Holzkoppel 4, D-22869 Schenefeld, Germany 24.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China 25.Carl von Ossietzky Univ Oldenburg, Dept Phys, D-26129 Oldenburg, Germany 26.Max Planck Inst Struktur & Dynam Mat, Luruper Chaussee 149, D-22761 Hamburg, Germany 27.Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany 28.PNDetector GmbH, Otto Hahn Ring, D-681739 Munich, Germany 29.Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging, Berkeley, CA 94720 USA 30.VA Med Ctr, Dept Radiat Oncol, Boston, MA 02130 USA 31.Phys Tech Bundesanstalt, Bundesallee 100, D-38116 Braunschweig, Germany 32.Lawrence Berkeley Natl Lab, Ctr Adv Math Energy Res Applicat, Berkeley, CA 94720 USA
推荐引用方式 GB/T 7714	Tanyag, Rico Mayro P.,Bacellar, Camila,Pang, Weiwu,et al. Sizes of pure and doped helium droplets from single shot x-ray imaging[J]. JOURNAL OF CHEMICAL PHYSICS,2022,156(4).
APA	Tanyag, Rico Mayro P..,Bacellar, Camila.,Pang, Weiwu.,Bernando, Charles.,Gomez, Luis F..,...&Vilesov, Andrey F..(2022).Sizes of pure and doped helium droplets from single shot x-ray imaging.JOURNAL OF CHEMICAL PHYSICS,156(4).
MLA	Tanyag, Rico Mayro P.,et al."Sizes of pure and doped helium droplets from single shot x-ray imaging".JOURNAL OF CHEMICAL PHYSICS 156.4(2022).