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Complete characterization of attosecond photoelectron wave packets
2021-11-23
发表期刊PHYSICAL REVIEW A (IF:2.6[JCR-2023],2.6[5-Year])
ISSN2469-9926
EISSN2469-9934
卷号104期号:5
DOI10.1103/PhysRevA.104.053526
摘要Development of attosecond laser technology allows us to measure electron dynamics such as photoionization delays between different species or electronic states. In general, the measured photoionization phase is a mixture of the spectral phase of the extreme ultraviolet (XUV) pulse and the atomic phases inherent to the optical transitions. Hence, it is difficult to disentangle these phases independently. Here we separate these phases by using an XUV attosecond pulse train containing both even and odd harmonic orders, generated by an 800and 400 nm laser pulse, in the presence of the infrared 800-nm pulse. We measure the photoelectron angular distributions as a function of two independently controlled delays, the XUV-IR and the 800-400 nm delays, with attosecond time resolution. We analyze the photoelectron angular distributions to determine the relative amplitudes and phases of each angular momentum component. Using an in situ technique, we determine the phases of the harmonic orders and thereby completely determine the atomic phases. Using the obtained atomic phases and amplitudes, we reconstruct the real and imaginary parts of the continuum wave functions associated with three individual photoionization pathways.
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收录类别SCIE ; EI
语种英语
WOS研究方向Optics ; Physics
WOS类目Optics ; Physics, Atomic, Molecular & Chemical
WOS记录号WOS:000722580100004
出版者AMER PHYSICAL SOC
原始文献类型Article
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文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/134162
专题大科学中心
物质科学与技术学院
通讯作者Niikura, Hiromichi
作者单位
1.CNR, Joint Attosecond Sci Lab, 100 Sussex Dr, Ottawa, ON K1A 0R6, Canada;
2.Univ Ottawa, 100 Sussex Dr, Ottawa, ON K1A 0R6, Canada;
3.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China;
4.Waseda Univ, Dept Appl Phys, Shinjyuku Ku, 3-4-1 Okubo, Tokyo 1698555, Japan
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GB/T 7714
Villeneuve, D. M.,Peng, Peng,Niikura, Hiromichi. Complete characterization of attosecond photoelectron wave packets[J]. PHYSICAL REVIEW A,2021,104(5).
APA Villeneuve, D. M.,Peng, Peng,&Niikura, Hiromichi.(2021).Complete characterization of attosecond photoelectron wave packets.PHYSICAL REVIEW A,104(5).
MLA Villeneuve, D. M.,et al."Complete characterization of attosecond photoelectron wave packets".PHYSICAL REVIEW A 104.5(2021).
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文件名: 10.1103@PhysRevA.104.053526.pdf
格式: Adobe PDF
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