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ShanghaiTech University Knowledge Management System
Complete characterization of attosecond photoelectron wave packets | |
2021-11-23 | |
发表期刊 | PHYSICAL REVIEW A (IF:2.6[JCR-2023],2.6[5-Year]) |
ISSN | 2469-9926 |
EISSN | 2469-9934 |
卷号 | 104期号:5 |
DOI | 10.1103/PhysRevA.104.053526 |
摘要 | Development of attosecond laser technology allows us to measure electron dynamics such as photoionization delays between different species or electronic states. In general, the measured photoionization phase is a mixture of the spectral phase of the extreme ultraviolet (XUV) pulse and the atomic phases inherent to the optical transitions. Hence, it is difficult to disentangle these phases independently. Here we separate these phases by using an XUV attosecond pulse train containing both even and odd harmonic orders, generated by an 800and 400 nm laser pulse, in the presence of the infrared 800-nm pulse. We measure the photoelectron angular distributions as a function of two independently controlled delays, the XUV-IR and the 800-400 nm delays, with attosecond time resolution. We analyze the photoelectron angular distributions to determine the relative amplitudes and phases of each angular momentum component. Using an in situ technique, we determine the phases of the harmonic orders and thereby completely determine the atomic phases. Using the obtained atomic phases and amplitudes, we reconstruct the real and imaginary parts of the continuum wave functions associated with three individual photoionization pathways. |
URL | 查看原文 |
收录类别 | SCIE ; EI |
语种 | 英语 |
WOS研究方向 | Optics ; Physics |
WOS类目 | Optics ; Physics, Atomic, Molecular & Chemical |
WOS记录号 | WOS:000722580100004 |
出版者 | AMER PHYSICAL SOC |
原始文献类型 | Article |
引用统计 | 正在获取...
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文献类型 | 期刊论文 |
条目标识符 | https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/134162 |
专题 | 大科学中心 物质科学与技术学院 |
通讯作者 | Niikura, Hiromichi |
作者单位 | 1.CNR, Joint Attosecond Sci Lab, 100 Sussex Dr, Ottawa, ON K1A 0R6, Canada; 2.Univ Ottawa, 100 Sussex Dr, Ottawa, ON K1A 0R6, Canada; 3.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China; 4.Waseda Univ, Dept Appl Phys, Shinjyuku Ku, 3-4-1 Okubo, Tokyo 1698555, Japan |
推荐引用方式 GB/T 7714 | Villeneuve, D. M.,Peng, Peng,Niikura, Hiromichi. Complete characterization of attosecond photoelectron wave packets[J]. PHYSICAL REVIEW A,2021,104(5). |
APA | Villeneuve, D. M.,Peng, Peng,&Niikura, Hiromichi.(2021).Complete characterization of attosecond photoelectron wave packets.PHYSICAL REVIEW A,104(5). |
MLA | Villeneuve, D. M.,et al."Complete characterization of attosecond photoelectron wave packets".PHYSICAL REVIEW A 104.5(2021). |
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