Sensitive Terahertz Detection and Imaging Driven by the Photothermoelectric Effect in Ultrashort-Channel Black Phosphorus Devices
2020-03
发表期刊ADVANCED SCIENCE (IF:14.3[JCR-2023],16.3[5-Year])
ISSN2198-3844
EISSN2198-3844
发表状态已发表
DOI10.1002/advs.201902699
摘要

Terahertz (THz) photon detection is of particular appealing for myriad applications, but it still lags behind efficient manipulation with electronics and photonics due to the lack of a suitable principle satisfying both high sensitivity and fast response at room temperature. Here, a new strategy is proposed to overcome these limitations by exploring the photothermoelectric (PTE) effect in an ultrashort (down to 30 nm) channel with black phosphorus as a photoactive material. The preferential flow of hot carriers is enabled by the asymmetric Cr/Au and Ti/Au metallization with the titled-angle evaporation technique. Most intriguingly, orders of magnitude field-enhancement beyond the skin-depth limit and photon absorption across a broadband frequency can be achieved. The PTE detector has excellent sensitivity of 297 V W-1, noise equivalent power less than 58 pW/Hz(0.5), and response time below 0.8 ms, which is superior to other thermal-based detectors at room temperature. A rigorous comparison with existing THz detectors, together with verification by further optical-pumping and imaging experiments, substantiates the importance of the localized field effect in the skin-depth limit. The results allow solid understanding on the role of PTE effect played in the THz photoresponse, opening up new opportunities for developing highly sensitive THz detectors for addressing targeted applications.

关键词black phosphorus imaging photothermoelectric effect terahertz detectors
收录类别SCI ; SCIE ; EI
语种英语
资助项目Zhejiang Provincial Natural Science Foundation[LQ20F050005]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science
WOS类目Chemistry, Multidisciplinary ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS记录号WOS:000507943700001
出版者WILEY
EI入藏号20200508116562
EI主题词Groundwater flow ; Imaging techniques ; Optical pumping ; Phosphorus
EI分类号Groundwater:444.2 ; Imaging Techniques:746 ; Chemical Products Generally:804 ; Atomic and Molecular Physics:931.3
WOS关键词GRAPHENE ; ELECTRONICS ; EFFICIENCY
原始文献类型Journal article (JA)
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文献类型期刊论文
条目标识符https://kms.shanghaitech.edu.cn/handle/2MSLDSTB/105174
专题物质科学与技术学院_硕士生
物质科学与技术学院_特聘教授组_陈效双组
物质科学与技术学院_特聘教授组_陆卫组
物质科学与技术学院_博士生
通讯作者Wang, Lin; Zhang, Kai; Chen, Xiaoshuang
作者单位
1.Chinese Acad Sci, Shanghai Inst Tech Phys, State Key Lab Infrared Phys, 500 Yu Tian Rd, Shanghai 200083, Peoples R China
2.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 100049, Peoples R China
3.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
4.Chinese Acad Sci, Suzhou Inst Nanotech & Nanobion SINANO, CAS Key Lab Nanobio Interface, Ruoshui Rd 398, Suzhou 215123, Jiangsu, Peoples R China
5.Chinese Acad Sci, Suzhou Inst Nanotech & Nanobion SINANO, Key Lab Nanodevices & Applicat, I Lab, Ruoshui Rd 398, Suzhou 215123, Jiangsu, Peoples R China
6.Univ Sci & Technol China, Sch Nano Technol & Nano Bion, Jinzhai Rd 96, Hefei 230026, Anhui, Peoples R China
7.Zhejiang Lab, 1818 Wenyixi Rd, Hangzhou 311100, Peoples R China
8.Fudan Univ, Inst Mol Mat & Devices, Dept Mat Sci, Shanghai 200433, Peoples R China
9.Fudan Univ, Dept Macromol Sci, Shanghai 200433, Peoples R China
第一作者单位物质科学与技术学院
通讯作者单位物质科学与技术学院
推荐引用方式
GB/T 7714
Guo, Wanlong,Dong, Zhuo,Xu, Yijun,et al. Sensitive Terahertz Detection and Imaging Driven by the Photothermoelectric Effect in Ultrashort-Channel Black Phosphorus Devices[J]. ADVANCED SCIENCE,2020.
APA Guo, Wanlong.,Dong, Zhuo.,Xu, Yijun.,Liu, Changlong.,Wei, Dacheng.,...&Lu, Wei.(2020).Sensitive Terahertz Detection and Imaging Driven by the Photothermoelectric Effect in Ultrashort-Channel Black Phosphorus Devices.ADVANCED SCIENCE.
MLA Guo, Wanlong,et al."Sensitive Terahertz Detection and Imaging Driven by the Photothermoelectric Effect in Ultrashort-Channel Black Phosphorus Devices".ADVANCED SCIENCE (2020).
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