Synergistic Improvements in Efficiency and Stability of 2D Perovskite Solar Cells with Metal Ion Doping
Xu, Qiaofei1,2,3; Meng, Ke1; Liu, Zhou1; Wang, Xiao1; Hu, Youdi1; Qiao, Zhi1; Li, Shunde1; Cheng, Lei1; Chen, Gang1,2,3
2019-11-11
Source PublicationADVANCED MATERIALS INTERFACES
ISSN2196-7350
Status已发表
DOI10.1002/admi.201901259
Abstract2D perovskites hold a great prospective to create highly efficient and stable solar cell devices. In order to explore their full potential, every component of 2D perovskite solar cells (PSCs) has to be carefully designed and engineered. Herein, the metal ion doping strategy is taken to optimize both the hole transport layers (HTLs) and the light absorbing layers of the BA(2)MA(3)Pb(4)I(13) (BA = butylamine; MA = methylammonium) based 2D PSC devices. The hole extraction and transport abilities are significantly enhanced by Cu ion doping in the nickel oxide layers, while the optoelectronic properties of the BA(2)MA(3)Pb(4)I(13) layers are effectively improved with Cs ion doping. The synergistic incorporations of Cu and Cs ions have boosted the device power conversion efficiency to 13.92%, the highest for 2D PSCs based on inorganic HTLs. In addition, the inorganic nature of the Cu doped nickel oxide film and the high quality of the Cs doped 2D perovskite film also endow the PSC device with extraordinary humidity and thermal stabilities.
Keyword2D perovskites metal ion doping solar cells stability
Indexed BySCI
Language英语
Funding ProjectScience and Technology Commission of Shanghai Municipality[17YF1412000] ; Science and Technology Commission of Shanghai Municipality[19ZR1476900]
WOS Research AreaChemistry ; Materials Science
WOS SubjectChemistry, Multidisciplinary ; Materials Science, Multidisciplinary
WOS IDWOS:000495492200001
PublisherWILEY
WOS KeywordHOLE-TRANSPORTING LAYER ; HIGH-PERFORMANCE ; HALIDE PEROVSKITES ; OPTICAL-PROPERTIES ; EXTRACTION ; ABSORBER ; CONTACT ; FILMS ; THIN
Original Document TypeArticle ; Early Access
Citation statistics
Cited Times [WOS]:0   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://kms.shanghaitech.edu.cn/handle/2MSLDSTB/102248
Collection物质科学与技术学院_硕士生
物质科学与技术学院_PI研究组_陈刚组
物质科学与技术学院_博士生
Corresponding AuthorChen, Gang
Affiliation1.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
2.Chinese Acad Sci, Shanghai Inst Ceram, Shanghai 200050, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
First Author AffilicationSchool of Physical Science and Technology
Corresponding Author AffilicationSchool of Physical Science and Technology
First Signature AffilicationSchool of Physical Science and Technology
Recommended Citation
GB/T 7714
Xu, Qiaofei,Meng, Ke,Liu, Zhou,et al. Synergistic Improvements in Efficiency and Stability of 2D Perovskite Solar Cells with Metal Ion Doping[J]. ADVANCED MATERIALS INTERFACES,2019.
APA Xu, Qiaofei.,Meng, Ke.,Liu, Zhou.,Wang, Xiao.,Hu, Youdi.,...&Chen, Gang.(2019).Synergistic Improvements in Efficiency and Stability of 2D Perovskite Solar Cells with Metal Ion Doping.ADVANCED MATERIALS INTERFACES.
MLA Xu, Qiaofei,et al."Synergistic Improvements in Efficiency and Stability of 2D Perovskite Solar Cells with Metal Ion Doping".ADVANCED MATERIALS INTERFACES (2019).
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